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Photocatalytic aerobic oxidation of toluene and its derivatives to aldehydes on Pd/Bi2WO6
Yuan, Bo1,2; Zhang, Bao1,2; Wang, Zhiliang1,2; Lu, Shengmei1; Li, Jun1; Liu, Yan1; Li, Can1
关键词Flower-like Bi2wo6 Toluene Oxidation Benzaldehyde Cocatalyst Palladium Nanoparticle
刊名CHINESE JOURNAL OF CATALYSIS
2017-03-01
DOI10.1016/S1872-2067(17)62757-8
38期:3页:440-446
收录类别SCI ; ISTP
文章类型Article
WOS标题词Science & Technology ; Physical Sciences ; Technology
类目[WOS]Chemistry, Applied ; Chemistry, Physical ; Engineering, Chemical
研究领域[WOS]Chemistry ; Engineering
关键词[WOS]GOLD NANOPARTICLES ; LIGHT ; EFFICIENT ; NANOSTRUCTURES ; BENZENE ; TIO2 ; CATALYSTS ; NB2O5
英文摘要The selective oxidation of toluene and its derivatives is extremely important in the chemical industry. The use of photocatalysis in organic synthesis has attracted considerable attention among synthetic chemists because of its "green" environmental characteristics. In this study, nanoscale Bi2WO6 with a flower-like morphology was found to be a highly efficient photocatalyst in the catalytic oxidation of toluene and its derivatives using O-2 as the oxidant. The loading of Pd nanoparticles as a cocatalyst onto the flower-like Bi2WO6 was found to produce a significant enhancement in the catalytic activity. Mechanistic investigation showed that the superior performance of Pd/Bi2WO6 could be attributed to the improvement of both the reductive and oxidative abilities of Bi2WO6 by the loading of the cocatalyst. (C) 2017, Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier B.V. All rights reserved.
语种英语
WOS记录号WOS:000400125100005
引用统计
被引频次:9[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/152013
专题中国科学院大连化学物理研究所
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Liaoning, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
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GB/T 7714
Yuan, Bo,Zhang, Bao,Wang, Zhiliang,et al. Photocatalytic aerobic oxidation of toluene and its derivatives to aldehydes on Pd/Bi2WO6[J]. CHINESE JOURNAL OF CATALYSIS,2017,38(3):440-446.
APA Yuan, Bo.,Zhang, Bao.,Wang, Zhiliang.,Lu, Shengmei.,Li, Jun.,...&Li, Can.(2017).Photocatalytic aerobic oxidation of toluene and its derivatives to aldehydes on Pd/Bi2WO6.CHINESE JOURNAL OF CATALYSIS,38(3),440-446.
MLA Yuan, Bo,et al."Photocatalytic aerobic oxidation of toluene and its derivatives to aldehydes on Pd/Bi2WO6".CHINESE JOURNAL OF CATALYSIS 38.3(2017):440-446.
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