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Tandem catalytic synthesis of benzene from CO2 and H-2
Zhu, Pengfei1,3; Sun, Jian2; Yang, Guohui3; Liu, Guoguo3; Zhang, Peipei3; Yoneyama, Yoshiharu3; Tsubaki, Noritatsu3
刊名CATALYSIS SCIENCE & TECHNOLOGY
2017-07-07
DOI10.1039/c7cy00842b
7页:2695-2699
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Chemistry, Physical
研究领域[WOS]Chemistry
关键词[WOS]METHANE DEHYDROAROMATIZATION ; NONOXIDATIVE CONDITIONS ; DEHYDRO-AROMATIZATION ; DIRECT CONVERSION ; CARBON OXIDES ; NATURAL-GAS ; MO/HZSM-5 ; ZEOLITE ; TEMPERATURE ; PERFORMANCE
英文摘要Benzene as an important raw material for production of industrial chemicals is generally synthesized from petroleum and coal tar. Here, we realized the synthesis of benzene from greenhouse CO2 and H-2 with two connected reactors by a tandem catalysis reaction comprising CO2 methanation and CH4 aromatization. The Ni/SiO2 catalyst loaded in the first reactor was used to convert CO2 to CH4, and the formed CH4 was sequentially converted to benzene on the Mo/HZSM-5 catalyst in the second reactor. The benzene formation rate reaches 0.68 mu molg(-1) min(-1) accompanied by a high CO2 conversion of 92%. This concept will provide a new pathway for the direct synthesis of benzene and CO2 utilization.
语种英语
WOS记录号WOS:000404887400004
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文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/152056
专题中国科学院大连化学物理研究所
作者单位1.Shaanxi Univ Sci & Technol, Sch Environm Sci & Engn, Xian 710021, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, Dalian 116023, Peoples R China
3.Univ Toyama, Sch Engn, Dept Appl Chem, Gofuku 3190, Toyama 9308555, Japan
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Zhu, Pengfei,Sun, Jian,Yang, Guohui,et al. Tandem catalytic synthesis of benzene from CO2 and H-2[J]. CATALYSIS SCIENCE & TECHNOLOGY,2017,7:2695-2699.
APA Zhu, Pengfei.,Sun, Jian.,Yang, Guohui.,Liu, Guoguo.,Zhang, Peipei.,...&Tsubaki, Noritatsu.(2017).Tandem catalytic synthesis of benzene from CO2 and H-2.CATALYSIS SCIENCE & TECHNOLOGY,7,2695-2699.
MLA Zhu, Pengfei,et al."Tandem catalytic synthesis of benzene from CO2 and H-2".CATALYSIS SCIENCE & TECHNOLOGY 7(2017):2695-2699.
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