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Iridium-Catalyzed Reductive Amination of Levulinic Acid to Pyrrolidinones under H-2 in Water
Xu, Zhanwei; Yan, Peifang; Jiang, Hong; Liu, Kairui; Zhang, Z. Conrad
关键词Iridium Reductive Amination Hydrogenation Levulinic Acid Biomass
刊名CHINESE JOURNAL OF CHEMISTRY
2017-05-01
DOI10.1002/cjoc.201600726
35页:581-585
收录类别SCI
文章类型Article
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Chemistry, Multidisciplinary
研究领域[WOS]Chemistry
关键词[WOS]FUNCTIONAL BIPYRIDONATE LIGAND ; GAMMA-VALEROLACTONE ; DEHYDROGENATIVE OXIDATION ; FORMIC-ACID ; TRANSFER HYDROGENATION ; CO2 HYDROGENATION ; COMPLEX BEARING ; AQUEOUS-MEDIA ; BIOMASS ; ALCOHOLS
英文摘要The synthesis of pyrrolidinones from reductive amination of levulinic acid (LA) with primary amines is reported. Pyrrolidinones have various applications such as surfactants, pharmaceutical intermediates, dispersants, and solvents. The half-sandwich Cp* Ir complex (Cp* is 1,2,3,4,5-pentamethylcyclopenta-1,3-diene) coordinated by bipyridine ligand bearing both dimethylamino and ortho-hydroxyl groups showed high catalytic activity for the reductive amination of LA. A range of primary amines, such as aromatic and benzyl amines, were readily converted to corresponding pyrrolidinones in good yields.
语种英语
WOS记录号WOS:000404028300009
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文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/152109
专题中国科学院大连化学物理研究所
作者单位Chinese Acad Sci, Dalian Natl Lab Clean Energy, State Key Lab Catalysis, Dalian Inst Chem Phys, Dalian 116023, Liaoning, Peoples R China
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Xu, Zhanwei,Yan, Peifang,Jiang, Hong,et al. Iridium-Catalyzed Reductive Amination of Levulinic Acid to Pyrrolidinones under H-2 in Water[J]. CHINESE JOURNAL OF CHEMISTRY,2017,35:581-585.
APA Xu, Zhanwei,Yan, Peifang,Jiang, Hong,Liu, Kairui,&Zhang, Z. Conrad.(2017).Iridium-Catalyzed Reductive Amination of Levulinic Acid to Pyrrolidinones under H-2 in Water.CHINESE JOURNAL OF CHEMISTRY,35,581-585.
MLA Xu, Zhanwei,et al."Iridium-Catalyzed Reductive Amination of Levulinic Acid to Pyrrolidinones under H-2 in Water".CHINESE JOURNAL OF CHEMISTRY 35(2017):581-585.
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