DICP OpenIR
Hydrides, Amides and Imides Mediated Ammonia Synthesis and Decomposition
Gao, Wenbo1,2; Guo, Jianping1,3; Chen, Ping1,3
Corresponding AuthorGuo, Jianping(guojianping@dicp.ac.cn) ; Chen, Ping(pchen@dicp.ac.cn)
Keywordammonia synthesis ammonia decomposition hydride imide amide
Source PublicationCHINESE JOURNAL OF CHEMISTRY
2019-05-01
ISSN1001-604X
DOI10.1002/cjoc.201800586
Volume37Issue:5Pages:442-451
Funding ProjectNational Natural Science Foundation of China[21633011] ; National Natural Science Foundation of China[21603220] ; National Natural Science Foundation of China[21872137] ; Sino-Japanese Research Cooperative Program of Ministry of Science and Technology[2016YFE0118300] ; DICP[DICP DMTO201504] ; Youth Innovation Promotion Association CAS[2018213] ; Collaborative Innovation Center of Chemistry for Energy Materials (2011-iChEM)
Funding OrganizationNational Natural Science Foundation of China ; National Natural Science Foundation of China ; Sino-Japanese Research Cooperative Program of Ministry of Science and Technology ; Sino-Japanese Research Cooperative Program of Ministry of Science and Technology ; DICP ; DICP ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; Collaborative Innovation Center of Chemistry for Energy Materials (2011-iChEM) ; Collaborative Innovation Center of Chemistry for Energy Materials (2011-iChEM) ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Sino-Japanese Research Cooperative Program of Ministry of Science and Technology ; Sino-Japanese Research Cooperative Program of Ministry of Science and Technology ; DICP ; DICP ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; Collaborative Innovation Center of Chemistry for Energy Materials (2011-iChEM) ; Collaborative Innovation Center of Chemistry for Energy Materials (2011-iChEM) ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Sino-Japanese Research Cooperative Program of Ministry of Science and Technology ; Sino-Japanese Research Cooperative Program of Ministry of Science and Technology ; DICP ; DICP ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; Collaborative Innovation Center of Chemistry for Energy Materials (2011-iChEM) ; Collaborative Innovation Center of Chemistry for Energy Materials (2011-iChEM) ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Sino-Japanese Research Cooperative Program of Ministry of Science and Technology ; Sino-Japanese Research Cooperative Program of Ministry of Science and Technology ; DICP ; DICP ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; Collaborative Innovation Center of Chemistry for Energy Materials (2011-iChEM) ; Collaborative Innovation Center of Chemistry for Energy Materials (2011-iChEM)
WOS SubjectChemistry, Multidisciplinary
WOS Research AreaChemistry
WOS KeywordMETAL NITRIDES ; MANGANESE NITRIDE ; NITROGEN TRANSFER ; HYDROGEN STORAGE ; CATALYSTS ; NH3 ; EFFICIENT ; N-2 ; RU ; GENERATION
AbstractAmmonia is feeding nearly half the world population and also holds the promise as a carbon-free energy carrier. The development of ammonia synthesis and decomposition processes under milder conditions is a grand challenge for more than a century. Increasing effort is devoted to this area in recent years and encouraging progress has been achieved. In this paper, we summarize our recent research using alkali or alkaline earth metal amides, imides and hydrides for ammonia synthesis and decomposition. These materials could serve as either indispensible component of active center in thermal catalytic process or nitrogen carrier for chemical looping ammonia synthesis. The synergy of amide, imide, or hydride with transition metals enables ammonia synthesis or decomposition with unprecedented high efficiency under milder reaction conditions, and thus opens an avenue to advance the chemistry or catalysis of N-2 fixation reaction. The compositional and structural diversity of the amide, imide and hydride materials provides plenty of opportunity and potential for further exploration and optimization.
Language英语
Funding OrganizationNational Natural Science Foundation of China ; National Natural Science Foundation of China ; Sino-Japanese Research Cooperative Program of Ministry of Science and Technology ; Sino-Japanese Research Cooperative Program of Ministry of Science and Technology ; DICP ; DICP ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; Collaborative Innovation Center of Chemistry for Energy Materials (2011-iChEM) ; Collaborative Innovation Center of Chemistry for Energy Materials (2011-iChEM) ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Sino-Japanese Research Cooperative Program of Ministry of Science and Technology ; Sino-Japanese Research Cooperative Program of Ministry of Science and Technology ; DICP ; DICP ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; Collaborative Innovation Center of Chemistry for Energy Materials (2011-iChEM) ; Collaborative Innovation Center of Chemistry for Energy Materials (2011-iChEM) ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Sino-Japanese Research Cooperative Program of Ministry of Science and Technology ; Sino-Japanese Research Cooperative Program of Ministry of Science and Technology ; DICP ; DICP ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; Collaborative Innovation Center of Chemistry for Energy Materials (2011-iChEM) ; Collaborative Innovation Center of Chemistry for Energy Materials (2011-iChEM) ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Sino-Japanese Research Cooperative Program of Ministry of Science and Technology ; Sino-Japanese Research Cooperative Program of Ministry of Science and Technology ; DICP ; DICP ; Youth Innovation Promotion Association CAS ; Youth Innovation Promotion Association CAS ; Collaborative Innovation Center of Chemistry for Energy Materials (2011-iChEM) ; Collaborative Innovation Center of Chemistry for Energy Materials (2011-iChEM)
WOS IDWOS:000466442600002
PublisherWILEY-V C H VERLAG GMBH
Citation statistics
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/165527
Collection中国科学院大连化学物理研究所
Corresponding AuthorGuo, Jianping; Chen, Ping
Affiliation1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, Dalian 116023, Liaoning, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.Collaborat Innovat Ctr Chem Energy Mat, Dalian 116023, Liaoning, Peoples R China
Recommended Citation
GB/T 7714
Gao, Wenbo,Guo, Jianping,Chen, Ping. Hydrides, Amides and Imides Mediated Ammonia Synthesis and Decomposition[J]. CHINESE JOURNAL OF CHEMISTRY,2019,37(5):442-451.
APA Gao, Wenbo,Guo, Jianping,&Chen, Ping.(2019).Hydrides, Amides and Imides Mediated Ammonia Synthesis and Decomposition.CHINESE JOURNAL OF CHEMISTRY,37(5),442-451.
MLA Gao, Wenbo,et al."Hydrides, Amides and Imides Mediated Ammonia Synthesis and Decomposition".CHINESE JOURNAL OF CHEMISTRY 37.5(2019):442-451.
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