DICP OpenIR
One-step preparation of phosphate-rich carbonaceous spheres via a hydrothermal approach for phosphopeptide analysis
Zhang, Haiyang1,2; Li, Xiaowei1,3; Ma, Shujuan1,2; Ou, Junjie1,3; Wei, Yinmao2; Ye, Mingliang1,3
Corresponding AuthorOu, Junjie(junjieou@dicp.ac.cn) ; Wei, Yinmao(ymwei@nwu.edu.cn)
Source PublicationGREEN CHEMISTRY
2019-04-21
ISSN1463-9262
DOI10.1039/c8gc03706j
Volume21Issue:8Pages:2052-2060
Funding ProjectChina State Key Basic Research Program Grant[2016YFA0501402] ; National Science Fund for Distinguished Young Scholars[21525524] ; National Natural Sciences Foundation of China[21575141] ; CAS-Weigao Research & Development Program[[2017]-009]
Funding OrganizationChina State Key Basic Research Program Grant ; China State Key Basic Research Program Grant ; National Science Fund for Distinguished Young Scholars ; National Science Fund for Distinguished Young Scholars ; National Natural Sciences Foundation of China ; National Natural Sciences Foundation of China ; CAS-Weigao Research & Development Program ; CAS-Weigao Research & Development Program ; China State Key Basic Research Program Grant ; China State Key Basic Research Program Grant ; National Science Fund for Distinguished Young Scholars ; National Science Fund for Distinguished Young Scholars ; National Natural Sciences Foundation of China ; National Natural Sciences Foundation of China ; CAS-Weigao Research & Development Program ; CAS-Weigao Research & Development Program ; China State Key Basic Research Program Grant ; China State Key Basic Research Program Grant ; National Science Fund for Distinguished Young Scholars ; National Science Fund for Distinguished Young Scholars ; National Natural Sciences Foundation of China ; National Natural Sciences Foundation of China ; CAS-Weigao Research & Development Program ; CAS-Weigao Research & Development Program ; China State Key Basic Research Program Grant ; China State Key Basic Research Program Grant ; National Science Fund for Distinguished Young Scholars ; National Science Fund for Distinguished Young Scholars ; National Natural Sciences Foundation of China ; National Natural Sciences Foundation of China ; CAS-Weigao Research & Development Program ; CAS-Weigao Research & Development Program
WOS SubjectChemistry, Multidisciplinary ; Green & Sustainable Science & Technology
WOS Research AreaChemistry ; Science & Technology - Other Topics
WOS KeywordHIGHLY SELECTIVE ENRICHMENT ; METAL-ORGANIC FRAMEWORK ; PHOSPHORYLATED PEPTIDES ; MONOLITHIC CAPILLARY ; FACILE PREPARATION ; MASS-SPECTROMETRY ; ENERGY-STORAGE ; IN-VIVO ; CARBONIZATION ; TITANIUM
AbstractCarbonaceous materials with different morphologies are attracting more and more attention in many fields due to their excellent performance. Various methods have been developed to prepare carbonaceous materials with different functions. In this work, we developed a green strategy to prepare phosphate-rich carbonaceous spheres via a one-step mild hydrothermal carbonization (HTC) process using glucose and vinylphosphonic acid (VPA) as precursors. Water was the sole solvent employed in this synthesis process, which is environmentally friendly. To augment the content of phosphate groups on the surfaces of carbonaceous spheres, water-soluble 4,4-azobis(4-cyanovaleric acid) was added to the HTC system as a thermal initiator. The size of the obtained carbonaceous spheres could reach 1-8 m. Following chelation with titanium ions (Ti4+), the carbonaceous spheres were applied as an immobilized metal affinity chromatography (IMAC) material; the Ti4+ content of carbonaceous spheres reached 2.685% (wt%). This synthetic process for Ti4+-IMAC carbonaceous spheres was facile and time-saving, avoiding the tedious and complex process for traditional Ti4+-IMAC materials. Furthermore, the Ti4+-IMAC carbonaceous spheres exhibited satisfactory enrichment ability for phosphopeptides in the digest of -casein and could enrich the low-abundance phosphopeptides in human serum, indicating a great potential use in phosphopeptide analysis.
Language英语
Funding OrganizationChina State Key Basic Research Program Grant ; China State Key Basic Research Program Grant ; National Science Fund for Distinguished Young Scholars ; National Science Fund for Distinguished Young Scholars ; National Natural Sciences Foundation of China ; National Natural Sciences Foundation of China ; CAS-Weigao Research & Development Program ; CAS-Weigao Research & Development Program ; China State Key Basic Research Program Grant ; China State Key Basic Research Program Grant ; National Science Fund for Distinguished Young Scholars ; National Science Fund for Distinguished Young Scholars ; National Natural Sciences Foundation of China ; National Natural Sciences Foundation of China ; CAS-Weigao Research & Development Program ; CAS-Weigao Research & Development Program ; China State Key Basic Research Program Grant ; China State Key Basic Research Program Grant ; National Science Fund for Distinguished Young Scholars ; National Science Fund for Distinguished Young Scholars ; National Natural Sciences Foundation of China ; National Natural Sciences Foundation of China ; CAS-Weigao Research & Development Program ; CAS-Weigao Research & Development Program ; China State Key Basic Research Program Grant ; China State Key Basic Research Program Grant ; National Science Fund for Distinguished Young Scholars ; National Science Fund for Distinguished Young Scholars ; National Natural Sciences Foundation of China ; National Natural Sciences Foundation of China ; CAS-Weigao Research & Development Program ; CAS-Weigao Research & Development Program
WOS IDWOS:000465398000020
PublisherROYAL SOC CHEMISTRY
Citation statistics
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/165599
Collection中国科学院大连化学物理研究所
Corresponding AuthorOu, Junjie; Wei, Yinmao
Affiliation1.Chinese Acad Sci, Key Lab Separat Sci Analyt Chem, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
2.Northwest Univ, Key Lab Synthet & Nat Funct Mol Chem, Minist Educ, Coll Chem & Mat Sci, Xian 710069, Shaanxi, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
Recommended Citation
GB/T 7714
Zhang, Haiyang,Li, Xiaowei,Ma, Shujuan,et al. One-step preparation of phosphate-rich carbonaceous spheres via a hydrothermal approach for phosphopeptide analysis[J]. GREEN CHEMISTRY,2019,21(8):2052-2060.
APA Zhang, Haiyang,Li, Xiaowei,Ma, Shujuan,Ou, Junjie,Wei, Yinmao,&Ye, Mingliang.(2019).One-step preparation of phosphate-rich carbonaceous spheres via a hydrothermal approach for phosphopeptide analysis.GREEN CHEMISTRY,21(8),2052-2060.
MLA Zhang, Haiyang,et al."One-step preparation of phosphate-rich carbonaceous spheres via a hydrothermal approach for phosphopeptide analysis".GREEN CHEMISTRY 21.8(2019):2052-2060.
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