DICP OpenIR
Crossed Beam Study on the F+D-2 -> DF+D Reaction at Hyperthermal Collision Energy of 23.84 kJ/mol
Wang, Hei-long1,2; Su, Shu2; Yu, Sheng-rui3; Che, Li1,4; Wu, Guo-rong2; Yuan, Kai-jun2; Yang, Xue-ming2; Minton, Timothy K.5
Corresponding AuthorChe, Li(liche@dlmu.edu.cn) ; Yuan, Kai-jun(kjyuan@dicp.ac.cn)
KeywordCrossed molecular beam Hyperthermal collision energy Rydberg tagging laser detonation
Source PublicationCHINESE JOURNAL OF CHEMICAL PHYSICS
2019-02-01
ISSN1674-0068
DOI10.1063/1674-0068/cjcp1901005
Volume32Issue:1Pages:151-156
Funding ProjectNational Natural Science Foundation of China[21473015] ; National Natural Science Foundation of China[21203016] ; National Natural Science Foundation of China[41574101] ; National Natural Science Foundation of China[21673232] ; National Natural Science Foundation of China[21773213] ; Foundation for the Author of National Excellent Doctoral Dissertation of China[201222]
Funding OrganizationNational Natural Science Foundation of China ; National Natural Science Foundation of China ; Foundation for the Author of National Excellent Doctoral Dissertation of China ; Foundation for the Author of National Excellent Doctoral Dissertation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Foundation for the Author of National Excellent Doctoral Dissertation of China ; Foundation for the Author of National Excellent Doctoral Dissertation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Foundation for the Author of National Excellent Doctoral Dissertation of China ; Foundation for the Author of National Excellent Doctoral Dissertation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Foundation for the Author of National Excellent Doctoral Dissertation of China ; Foundation for the Author of National Excellent Doctoral Dissertation of China
WOS SubjectPhysics, Atomic, Molecular & Chemical
WOS Research AreaPhysics
WOS KeywordMOLECULAR-BEAM ; ATOMIC-OXYGEN ; F PLUS ; ANGULAR-DISTRIBUTIONS ; SCATTERING DYNAMICS ; REACTION F+D-2 ; STATE ; SECTIONS ; SURFACE ; RESONANCES
AbstractWe presented an experimental apparatus combining the H-atom Rydberg tagging time-of-flight technique and the laser detonation source for studying crossed beam reactions at hyperthermal collision energies. The preliminary study of the F+D-2 -> DF+D reaction at hyperthermal collision energy of 23.84 kJ/mol was performed. Two beam sources were used in this study: one is the hyperthermal F beam source produced by a laser detonation process, and the other is D-2 beam source generated by liquid-N-2 cooled pulsed valve. Vibrational state-resolved differential cross sections (DCSs) of product for the title reaction were determined. From the product vibrational state-resolved DCS, it can be concluded that products DF(v' =0, 1, 2, 3) are predominantly distributed in the sideway and backward scattering directions at this collision energy. However, the highest vibrational excited product DF(v'=4), is clearly peaked in the forward direction. The probable dynamical origins for these forward scattering products were analyzed and discussed.
Language英语
Funding OrganizationNational Natural Science Foundation of China ; National Natural Science Foundation of China ; Foundation for the Author of National Excellent Doctoral Dissertation of China ; Foundation for the Author of National Excellent Doctoral Dissertation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Foundation for the Author of National Excellent Doctoral Dissertation of China ; Foundation for the Author of National Excellent Doctoral Dissertation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Foundation for the Author of National Excellent Doctoral Dissertation of China ; Foundation for the Author of National Excellent Doctoral Dissertation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Foundation for the Author of National Excellent Doctoral Dissertation of China ; Foundation for the Author of National Excellent Doctoral Dissertation of China
WOS IDWOS:000461781200021
PublisherCHINESE PHYSICAL SOC
Citation statistics
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/165835
Collection中国科学院大连化学物理研究所
Corresponding AuthorChe, Li; Yuan, Kai-jun
Affiliation1.Dalian Maritime Univ, Coll Environm Sci & Engn, Dalian 116026, Peoples R China
2.Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China
3.Zhejiang Normal Univ, Hangzhou Inst Adv Studies, Hangzhou 311231, Zhejiang, Peoples R China
4.Dalian Maritime Univ, Coll Sci, Dalian 116026, Peoples R China
5.Montana State Univ, Dept Chem & Biochem, Bozeman, MT 59717 USA
Recommended Citation
GB/T 7714
Wang, Hei-long,Su, Shu,Yu, Sheng-rui,et al. Crossed Beam Study on the F+D-2 -> DF+D Reaction at Hyperthermal Collision Energy of 23.84 kJ/mol[J]. CHINESE JOURNAL OF CHEMICAL PHYSICS,2019,32(1):151-156.
APA Wang, Hei-long.,Su, Shu.,Yu, Sheng-rui.,Che, Li.,Wu, Guo-rong.,...&Minton, Timothy K..(2019).Crossed Beam Study on the F+D-2 -> DF+D Reaction at Hyperthermal Collision Energy of 23.84 kJ/mol.CHINESE JOURNAL OF CHEMICAL PHYSICS,32(1),151-156.
MLA Wang, Hei-long,et al."Crossed Beam Study on the F+D-2 -> DF+D Reaction at Hyperthermal Collision Energy of 23.84 kJ/mol".CHINESE JOURNAL OF CHEMICAL PHYSICS 32.1(2019):151-156.
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