DICP OpenIR
Application of In Situ Techniques for the Characterization of NiFe-Based Oxygen Evolution Reaction (OER) Electrocatalysts
Zhu, Kaiyue1,2; Zhu, Xuefeng1; Yang, Weishen1
Corresponding AuthorZhu, Xuefeng(zhuxf@dicp.ac.cn) ; Yang, Weishen(yangws@dicp.ac.cn)
Keywordactive centers in situ techniques intermediates NiFe-based electrocatalysts oxygen evolution reaction
Source PublicationANGEWANDTE CHEMIE-INTERNATIONAL EDITION
2019-01-28
ISSN1433-7851
DOI10.1002/anie.201802923
Volume58Issue:5Pages:1252-1265
Funding ProjectNational Natural Science Foundation of China[91545202] ; National Natural Science Foundation of China[U1508203] ; National Natural Science Foundation of China[21776267] ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS)[XDB17000000] ; project of Dalian Outstanding Young Scientific and Technical Talents[2016RJ07] ; Youth Innovation Promotion Association of CAS[2014161]
Funding OrganizationNational Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; project of Dalian Outstanding Young Scientific and Technical Talents ; project of Dalian Outstanding Young Scientific and Technical Talents ; Youth Innovation Promotion Association of CAS ; Youth Innovation Promotion Association of CAS ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; project of Dalian Outstanding Young Scientific and Technical Talents ; project of Dalian Outstanding Young Scientific and Technical Talents ; Youth Innovation Promotion Association of CAS ; Youth Innovation Promotion Association of CAS ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; project of Dalian Outstanding Young Scientific and Technical Talents ; project of Dalian Outstanding Young Scientific and Technical Talents ; Youth Innovation Promotion Association of CAS ; Youth Innovation Promotion Association of CAS ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; project of Dalian Outstanding Young Scientific and Technical Talents ; project of Dalian Outstanding Young Scientific and Technical Talents ; Youth Innovation Promotion Association of CAS ; Youth Innovation Promotion Association of CAS
WOS SubjectChemistry, Multidisciplinary
WOS Research AreaChemistry
WOS KeywordRAY-ABSORPTION SPECTROSCOPY ; WATER-OXIDATION ; OXYHYDROXIDE ELECTROCATALYSTS ; ELECTROCHEMICAL EVOLUTION ; ELECTRONIC-STRUCTURE ; RAMAN-SPECTROSCOPY ; ENERGY-CONVERSION ; REACTION DYNAMICS ; AIR BATTERIES ; REDOX STATES
AbstractDeveloping high-efficiency and affordable electrocatalysts for the sluggish oxygen evolution reaction (OER) remains a crucial bottleneck on the way to the practical applications of rechargeable energy storage technologies and water splitting for producing clean fuel (H-2). In recent years, NiFe-based materials have proven to be excellent electrocatalysts for OER. Understanding the characteristics that affect OER activity and determining the OER mechanism are of vital importance for the development of OER electrocatalysts. Therefore, in situ characterization techniques performed under OER conditions are urgently needed to monitor the key intermediates together with identifying the OER active centers and phases. In this Minireview, recent advances regarding in situ techniques for the characterization of NiFe-based electrocatalysts are thoroughly summarized, including Raman spectroscopy, X-ray absorption spectroscopy, ambient pressure X-ray photoelectron spectroscopy, Mcssbauer spectroscopy, Ultraviolet-visible spectroscopy, differential electrochemical mass spectrometry, and surface interrogation scanning electrochemical microscopy. The results from these in situ measurements not only reveal the structural transformation and the progressive oxidation of the catalytic species under OER conditions, but also disclose the crucial role of Ni and Fe during the OER. Finally, the need for developing new in situ techniques and theoretical investigations is discussed to better understand the OER mechanism and design promising OER electrocatalysts.
Language英语
Funding OrganizationNational Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; project of Dalian Outstanding Young Scientific and Technical Talents ; project of Dalian Outstanding Young Scientific and Technical Talents ; Youth Innovation Promotion Association of CAS ; Youth Innovation Promotion Association of CAS ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; project of Dalian Outstanding Young Scientific and Technical Talents ; project of Dalian Outstanding Young Scientific and Technical Talents ; Youth Innovation Promotion Association of CAS ; Youth Innovation Promotion Association of CAS ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; project of Dalian Outstanding Young Scientific and Technical Talents ; project of Dalian Outstanding Young Scientific and Technical Talents ; Youth Innovation Promotion Association of CAS ; Youth Innovation Promotion Association of CAS ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; project of Dalian Outstanding Young Scientific and Technical Talents ; project of Dalian Outstanding Young Scientific and Technical Talents ; Youth Innovation Promotion Association of CAS ; Youth Innovation Promotion Association of CAS
WOS IDWOS:000458826100002
PublisherWILEY-V C H VERLAG GMBH
Citation statistics
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/166007
Collection中国科学院大连化学物理研究所
Corresponding AuthorZhu, Xuefeng; Yang, Weishen
Affiliation1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, 457 Zhongshan Rd, Dalian 116023, Liaoning, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
Recommended Citation
GB/T 7714
Zhu, Kaiyue,Zhu, Xuefeng,Yang, Weishen. Application of In Situ Techniques for the Characterization of NiFe-Based Oxygen Evolution Reaction (OER) Electrocatalysts[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2019,58(5):1252-1265.
APA Zhu, Kaiyue,Zhu, Xuefeng,&Yang, Weishen.(2019).Application of In Situ Techniques for the Characterization of NiFe-Based Oxygen Evolution Reaction (OER) Electrocatalysts.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,58(5),1252-1265.
MLA Zhu, Kaiyue,et al."Application of In Situ Techniques for the Characterization of NiFe-Based Oxygen Evolution Reaction (OER) Electrocatalysts".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION 58.5(2019):1252-1265.
Files in This Item:
There are no files associated with this item.
Related Services
Recommend this item
Bookmark
Usage statistics
Export to Endnote
Google Scholar
Similar articles in Google Scholar
[Zhu, Kaiyue]'s Articles
[Zhu, Xuefeng]'s Articles
[Yang, Weishen]'s Articles
Baidu academic
Similar articles in Baidu academic
[Zhu, Kaiyue]'s Articles
[Zhu, Xuefeng]'s Articles
[Yang, Weishen]'s Articles
Bing Scholar
Similar articles in Bing Scholar
[Zhu, Kaiyue]'s Articles
[Zhu, Xuefeng]'s Articles
[Yang, Weishen]'s Articles
Terms of Use
No data!
Social Bookmark/Share
All comments (0)
No comment.
 

Items in the repository are protected by copyright, with all rights reserved, unless otherwise indicated.