DICP OpenIR
Toward Fundamentals of Confined Electrocatalysis in Nanoscale Reactors
Li, Haobo1; Guo, Chenxi1; Fu, Qiang2; Xiao, Jianping1,2
Corresponding AuthorXiao, Jianping(xiao@dicp.ac.cn)
Source PublicationJOURNAL OF PHYSICAL CHEMISTRY LETTERS
2019-02-07
ISSN1948-7185
DOI10.1021/acs.jpclett.8b03448
Volume10Issue:3Pages:533-539
Funding ProjectNational Science Foundation of China[21802124] ; National Science Foundation of China[91845103] ; Ministry of Science and Technology of China[2016YFA0200200] ; Strategic Priority Research Program of the Chinese Academy of Sciences[XDB17020000]
Funding OrganizationNational Science Foundation of China ; National Science Foundation of China ; Ministry of Science and Technology of China ; Ministry of Science and Technology of China ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; National Science Foundation of China ; National Science Foundation of China ; Ministry of Science and Technology of China ; Ministry of Science and Technology of China ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; National Science Foundation of China ; National Science Foundation of China ; Ministry of Science and Technology of China ; Ministry of Science and Technology of China ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; National Science Foundation of China ; National Science Foundation of China ; Ministry of Science and Technology of China ; Ministry of Science and Technology of China ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences
WOS SubjectChemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Atomic, Molecular & Chemical
WOS Research AreaChemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
WOS KeywordGRAPHENE FILMS ; CATALYSIS ; POINTS ; SIZE
AbstractA number of experiments have demonstrated that electrochemical reactions are feasible in confined nanoscale reactors, while what the fundamentals of confined electrochemistry are is not clear. Using first-principles calculations and electrochemical modeling, we find that the capacitance in the confined nanoscale reactors can be significantly enhanced, compared to an open electrode interface, essentially promoting the electrochemical reactions and charge transfer efficiency in nanoscale reactors. More importantly, this is a general character, as found in a variety of electrochemical and thermochemical reactions. At the end, we use the recently defined new concept of "confinement energy" for understanding the nature of confined electrochemistry from both thermochemical and electrochemical points of view.
Language英语
Funding OrganizationNational Science Foundation of China ; National Science Foundation of China ; Ministry of Science and Technology of China ; Ministry of Science and Technology of China ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; National Science Foundation of China ; National Science Foundation of China ; Ministry of Science and Technology of China ; Ministry of Science and Technology of China ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; National Science Foundation of China ; National Science Foundation of China ; Ministry of Science and Technology of China ; Ministry of Science and Technology of China ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; National Science Foundation of China ; National Science Foundation of China ; Ministry of Science and Technology of China ; Ministry of Science and Technology of China ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences
WOS IDWOS:000458704800035
PublisherAMER CHEMICAL SOC
Citation statistics
Cited Times:1[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/166045
Collection中国科学院大连化学物理研究所
Corresponding AuthorXiao, Jianping
Affiliation1.Westlake Univ, Sch Sci, Westlake Inst Adv Study, Inst Nat Sci, Hangzhou 310024, Zhejiang, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Zhongshan Rd 457, Dalian 116023, Peoples R China
Recommended Citation
GB/T 7714
Li, Haobo,Guo, Chenxi,Fu, Qiang,et al. Toward Fundamentals of Confined Electrocatalysis in Nanoscale Reactors[J]. JOURNAL OF PHYSICAL CHEMISTRY LETTERS,2019,10(3):533-539.
APA Li, Haobo,Guo, Chenxi,Fu, Qiang,&Xiao, Jianping.(2019).Toward Fundamentals of Confined Electrocatalysis in Nanoscale Reactors.JOURNAL OF PHYSICAL CHEMISTRY LETTERS,10(3),533-539.
MLA Li, Haobo,et al."Toward Fundamentals of Confined Electrocatalysis in Nanoscale Reactors".JOURNAL OF PHYSICAL CHEMISTRY LETTERS 10.3(2019):533-539.
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