DICP OpenIR
Dual-phase membrane reactor for hydrogen separation with high tolerance to CO2 and H2S impurities
Cai, Lili1,2; Hu, Shiqing1,2; Cao, Zhongwei1; Li, Hongbo1; Zhu, Xuefeng1; Yang, Weishen1
Corresponding AuthorZhu, Xuefeng(zhuxf@dicp.ac.cn) ; Yang, Weishen(yangws@dicp.ac.cn)
Keywordhydrogen separation oxygen-permeable membranes membrane reactor conductivity CO2 and H2S impurities
Source PublicationAICHE JOURNAL
2019-03-01
ISSN0001-1541
DOI10.1002/aic.16491
Volume65Issue:3Pages:1088-1096
Funding ProjectNational Natural Science Foundation of China[91545202] ; National Natural Science Foundation of China[21776267] ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS)[XDB17000000] ; project of Dalian Outstanding Young Scientific and Technical Talents[2016RJ07] ; Dalian National Laboratory for Clean Energy (DNL), CAS ; DICPQIBEBT[UN201708] ; DICP[DMTO201503]
Funding OrganizationNational Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; project of Dalian Outstanding Young Scientific and Technical Talents ; project of Dalian Outstanding Young Scientific and Technical Talents ; Dalian National Laboratory for Clean Energy (DNL), CAS ; Dalian National Laboratory for Clean Energy (DNL), CAS ; DICPQIBEBT ; DICPQIBEBT ; DICP ; DICP ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; project of Dalian Outstanding Young Scientific and Technical Talents ; project of Dalian Outstanding Young Scientific and Technical Talents ; Dalian National Laboratory for Clean Energy (DNL), CAS ; Dalian National Laboratory for Clean Energy (DNL), CAS ; DICPQIBEBT ; DICPQIBEBT ; DICP ; DICP ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; project of Dalian Outstanding Young Scientific and Technical Talents ; project of Dalian Outstanding Young Scientific and Technical Talents ; Dalian National Laboratory for Clean Energy (DNL), CAS ; Dalian National Laboratory for Clean Energy (DNL), CAS ; DICPQIBEBT ; DICPQIBEBT ; DICP ; DICP ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; project of Dalian Outstanding Young Scientific and Technical Talents ; project of Dalian Outstanding Young Scientific and Technical Talents ; Dalian National Laboratory for Clean Energy (DNL), CAS ; Dalian National Laboratory for Clean Energy (DNL), CAS ; DICPQIBEBT ; DICPQIBEBT ; DICP ; DICP
WOS SubjectEngineering, Chemical
WOS Research AreaEngineering
WOS KeywordHOLLOW-FIBER MEMBRANE ; OXYGEN PERMEATION ; PARTIAL OXIDATION ; FUEL-CELL ; COMPOSITE ; ELECTROCATALYSTS ; METHANE ; DESIGN ; SYNGAS ; SYSTEM
AbstractCatalytic membrane reactors based on oxygen-permeable membranes are recently studied for hydrogen separation because their hydrogen separation rates and separation factors are comparable to those of Pd-based membranes. New membrane materials with high performance and good tolerance to CO2 and H2S impurities are highly desired. In this work, a new membrane material Ce0.85Sm0.15O1.925-Sr2Fe1.5Mo0.5O6-delta (SDC-SFM) was prepared for hydrogen separation. It exhibits high conductivities at low oxygen partial pressures, which is benefit to electron transfer and ion diffusion. A high hydrogen separation rate of 6.6 mL cm(-2) min(-1) was obtained on a 0.5-mm-thick membrane coated with Ni/SDC catalyst at 900 degrees C. The membrane reactor was operated steadily for 532 h under atmospheres containing CO2 and H2S impurities. Various characterizations reveal that SDC-SFM has good stability in the membrane reactor for hydrogen separation. All facts confirm that SDC-SFM is promising for hydrogen separation in practical applications. (c) 2018 American Institute of Chemical Engineers
Language英语
Funding OrganizationNational Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; project of Dalian Outstanding Young Scientific and Technical Talents ; project of Dalian Outstanding Young Scientific and Technical Talents ; Dalian National Laboratory for Clean Energy (DNL), CAS ; Dalian National Laboratory for Clean Energy (DNL), CAS ; DICPQIBEBT ; DICPQIBEBT ; DICP ; DICP ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; project of Dalian Outstanding Young Scientific and Technical Talents ; project of Dalian Outstanding Young Scientific and Technical Talents ; Dalian National Laboratory for Clean Energy (DNL), CAS ; Dalian National Laboratory for Clean Energy (DNL), CAS ; DICPQIBEBT ; DICPQIBEBT ; DICP ; DICP ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; project of Dalian Outstanding Young Scientific and Technical Talents ; project of Dalian Outstanding Young Scientific and Technical Talents ; Dalian National Laboratory for Clean Energy (DNL), CAS ; Dalian National Laboratory for Clean Energy (DNL), CAS ; DICPQIBEBT ; DICPQIBEBT ; DICP ; DICP ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; project of Dalian Outstanding Young Scientific and Technical Talents ; project of Dalian Outstanding Young Scientific and Technical Talents ; Dalian National Laboratory for Clean Energy (DNL), CAS ; Dalian National Laboratory for Clean Energy (DNL), CAS ; DICPQIBEBT ; DICPQIBEBT ; DICP ; DICP
WOS IDWOS:000457747600020
PublisherWILEY
Citation statistics
Cited Times:1[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/166063
Collection中国科学院大连化学物理研究所
Corresponding AuthorZhu, Xuefeng; Yang, Weishen
Affiliation1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
Recommended Citation
GB/T 7714
Cai, Lili,Hu, Shiqing,Cao, Zhongwei,et al. Dual-phase membrane reactor for hydrogen separation with high tolerance to CO2 and H2S impurities[J]. AICHE JOURNAL,2019,65(3):1088-1096.
APA Cai, Lili,Hu, Shiqing,Cao, Zhongwei,Li, Hongbo,Zhu, Xuefeng,&Yang, Weishen.(2019).Dual-phase membrane reactor for hydrogen separation with high tolerance to CO2 and H2S impurities.AICHE JOURNAL,65(3),1088-1096.
MLA Cai, Lili,et al."Dual-phase membrane reactor for hydrogen separation with high tolerance to CO2 and H2S impurities".AICHE JOURNAL 65.3(2019):1088-1096.
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