DICP OpenIR
Asymmetric dual-phase MIEC membrane reactor for energy-efficient coproduction of two kinds of synthesis gases
Li, Wenping1,2; Cao, Zhongwei1; Li, Hongbo1; Zhu, Xuefeng1; Yang, Weishen1
Corresponding AuthorZhu, Xuefeng(zhuxf@dicp.ac.cn)
KeywordAsymmetric dual-phase membrane Membrane reactor Ammonia synthesis gas Liquid fuels synthesis gas Partial oxidation of methane Water splitting
Source PublicationINTERNATIONAL JOURNAL OF HYDROGEN ENERGY
2019-02-08
ISSN0360-3199
DOI10.1016/j.ijhydene.2018.12.182
Volume44Issue:8Pages:4218-4227
Funding ProjectNational Natural Science Foundation of China[91545202] ; National Natural Science Foundation of China[U1508203] ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS)[XDB17000000] ; project of Dalian Outstanding Young Scientific and Technical Talents[2016RJ07] ; DICP[DICP DMTO201503]
Funding OrganizationNational Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; project of Dalian Outstanding Young Scientific and Technical Talents ; project of Dalian Outstanding Young Scientific and Technical Talents ; DICP ; DICP ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; project of Dalian Outstanding Young Scientific and Technical Talents ; project of Dalian Outstanding Young Scientific and Technical Talents ; DICP ; DICP ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; project of Dalian Outstanding Young Scientific and Technical Talents ; project of Dalian Outstanding Young Scientific and Technical Talents ; DICP ; DICP ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; project of Dalian Outstanding Young Scientific and Technical Talents ; project of Dalian Outstanding Young Scientific and Technical Talents ; DICP ; DICP
WOS SubjectChemistry, Physical ; Electrochemistry ; Energy & Fuels
WOS Research AreaChemistry ; Electrochemistry ; Energy & Fuels
WOS KeywordOXYGEN PERMEATION PROPERTIES ; PARTIAL OXIDATION ; CERAMIC MEMBRANES ; METHANE ; WATER ; SEPARATION ; SYNGAS ; PERFORMANCE ; PEROVSKITE ; HYDROGEN
AbstractAn asymmetric 75 wt% Sm0.15Ce0.85O1.925-25 wt% Sm0.6Sr0.4Al0.3Fe0.7O3-delta (SDC-SSAF) dual-phase mixed ionic-electronic conducting (MIEC) oxygen-permeable membrane reactor was applied to coproduce ammonia synthesis gas (ASG, H-2/N-2 = 3) and liquid fuels synthesis gas (LFSG, H-2/CO = 2). The effects of CH4 concentration, CH4 flow rate, steam flow rate and temperature on the performance of the membrane reactor were studied. The SDC-SSAF membrane reactor showed an excellent performance for the coproduction of ASG and LFSG. An ASG production rate of 20.7 mL cm(-2) min(-1), a LFSG production rate of 51.0 mL cm(-2) min(-1) and an oxygen permeation rate of 9.1 mL cm(-2) min(-1) were achieved at 925 degrees C. Compared with traditional industrial processes, the energy saving of this membrane reactor process is expected as high as 66.5%. The post-mortem of the membrane reactor using scanning electron microscope (SEM) and energy dispersive spectroscopy (EDS) characterization revealed that the membrane has an excellent structural stability under operation condition.
Language英语
Funding OrganizationNational Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; project of Dalian Outstanding Young Scientific and Technical Talents ; project of Dalian Outstanding Young Scientific and Technical Talents ; DICP ; DICP ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; project of Dalian Outstanding Young Scientific and Technical Talents ; project of Dalian Outstanding Young Scientific and Technical Talents ; DICP ; DICP ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; project of Dalian Outstanding Young Scientific and Technical Talents ; project of Dalian Outstanding Young Scientific and Technical Talents ; DICP ; DICP ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; Strategic Priority Research Program of the Chinese Academy of Sciences (CAS) ; project of Dalian Outstanding Young Scientific and Technical Talents ; project of Dalian Outstanding Young Scientific and Technical Talents ; DICP ; DICP
WOS IDWOS:000458224700020
PublisherPERGAMON-ELSEVIER SCIENCE LTD
Citation statistics
Cited Times:2[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/166099
Collection中国科学院大连化学物理研究所
Corresponding AuthorZhu, Xuefeng
Affiliation1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
Recommended Citation
GB/T 7714
Li, Wenping,Cao, Zhongwei,Li, Hongbo,et al. Asymmetric dual-phase MIEC membrane reactor for energy-efficient coproduction of two kinds of synthesis gases[J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,2019,44(8):4218-4227.
APA Li, Wenping,Cao, Zhongwei,Li, Hongbo,Zhu, Xuefeng,&Yang, Weishen.(2019).Asymmetric dual-phase MIEC membrane reactor for energy-efficient coproduction of two kinds of synthesis gases.INTERNATIONAL JOURNAL OF HYDROGEN ENERGY,44(8),4218-4227.
MLA Li, Wenping,et al."Asymmetric dual-phase MIEC membrane reactor for energy-efficient coproduction of two kinds of synthesis gases".INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 44.8(2019):4218-4227.
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