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Coherent interference of molecular electronic states in NO by two-color femtosecond laser pulses
Hu, Wenhui1; Liu, Yong2; Luo, Sizuo1; Li, Xing1; Yu, Jiaqi1; Li, Xiaokai1; Sun, Zhigang2; Yuan, Kai-Jun1,3; Bandrauk, Andre D.3; Ding, Dajun1
Corresponding AuthorLuo, Sizuo(luosz@jlu.edu.cn) ; Yuan, Kai-Jun(kaijun.yuan@usherbrooke.ca) ; Ding, Dajun(dajund@jlu.edu.cn)
Source PublicationPHYSICAL REVIEW A
2019-01-22
ISSN2469-9926
DOI10.1103/PhysRevA.99.011402
Volume99Issue:1Pages:6
Funding ProjectNational Natural Science Foundation of China (NNSFC)[11704148] ; National Natural Science Foundation of China (NNSFC)[11534004] ; National Natural Science Foundation of China (NNSFC)[11627807] ; National Natural Science Foundation of China (NNSFC)[21222308] ; National Natural Science Foundation of China (NNSFC)[21133006] ; National Natural Science Foundation of China (NNSFC)[21433009] ; China Postdoctoral Science Foundation[2015M571336] ; NSERC ; FQRNT
Funding OrganizationNational Natural Science Foundation of China (NNSFC) ; National Natural Science Foundation of China (NNSFC) ; China Postdoctoral Science Foundation ; China Postdoctoral Science Foundation ; NSERC ; NSERC ; FQRNT ; FQRNT ; National Natural Science Foundation of China (NNSFC) ; National Natural Science Foundation of China (NNSFC) ; China Postdoctoral Science Foundation ; China Postdoctoral Science Foundation ; NSERC ; NSERC ; FQRNT ; FQRNT ; National Natural Science Foundation of China (NNSFC) ; National Natural Science Foundation of China (NNSFC) ; China Postdoctoral Science Foundation ; China Postdoctoral Science Foundation ; NSERC ; NSERC ; FQRNT ; FQRNT ; National Natural Science Foundation of China (NNSFC) ; National Natural Science Foundation of China (NNSFC) ; China Postdoctoral Science Foundation ; China Postdoctoral Science Foundation ; NSERC ; NSERC ; FQRNT ; FQRNT
WOS SubjectOptics ; Physics, Atomic, Molecular & Chemical
WOS Research AreaOptics ; Physics
WOS KeywordCIRCULAR-DICHROISM ; DYNAMICS ; PHOTOELECTRON ; DIFFRACTION ; IONIZATION ; MIGRATION ; BREAKING
AbstractQuantum coherence interference between electronic states in molecules is an important factor for controlling electronic and nuclear dynamics in photoinduced physics and chemistry. We measure and model molecular angle-dependent photoionization yields to explore coherent interference dynamics between quasiequal energy electronic-vibrational states of the nitric oxide molecule, NO, by ultrafast phase-controlled two-color femtosecond laser pulses. We demonstrate by experiment and theory that the photoelectron angular distribution of NO, where two excited electronic states are coherently combined by ultrafast pulses, is a function of the relative phase of the pulses, and the photoelectron kinetic energy. The modification of photoelectron emission angular patterns encodes the information of the coherence via electronic state interference. The result allows access to phase-dependent state correlations and ultrafast vibrationic dynamics in molecules.
Language英语
Funding OrganizationNational Natural Science Foundation of China (NNSFC) ; National Natural Science Foundation of China (NNSFC) ; China Postdoctoral Science Foundation ; China Postdoctoral Science Foundation ; NSERC ; NSERC ; FQRNT ; FQRNT ; National Natural Science Foundation of China (NNSFC) ; National Natural Science Foundation of China (NNSFC) ; China Postdoctoral Science Foundation ; China Postdoctoral Science Foundation ; NSERC ; NSERC ; FQRNT ; FQRNT ; National Natural Science Foundation of China (NNSFC) ; National Natural Science Foundation of China (NNSFC) ; China Postdoctoral Science Foundation ; China Postdoctoral Science Foundation ; NSERC ; NSERC ; FQRNT ; FQRNT ; National Natural Science Foundation of China (NNSFC) ; National Natural Science Foundation of China (NNSFC) ; China Postdoctoral Science Foundation ; China Postdoctoral Science Foundation ; NSERC ; NSERC ; FQRNT ; FQRNT
WOS IDWOS:000456287500003
PublisherAMER PHYSICAL SOC
Citation statistics
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/166293
Collection中国科学院大连化学物理研究所
Corresponding AuthorLuo, Sizuo; Yuan, Kai-Jun; Ding, Dajun
Affiliation1.Jilin Univ, Inst Atom & Mol Phys, Changchun 130012, Jilin, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China
3.Univ Sherbrooke, Fac Sci, Lab Chim Theor, Sherbrooke, PQ J1K 2R1, Canada
Recommended Citation
GB/T 7714
Hu, Wenhui,Liu, Yong,Luo, Sizuo,et al. Coherent interference of molecular electronic states in NO by two-color femtosecond laser pulses[J]. PHYSICAL REVIEW A,2019,99(1):6.
APA Hu, Wenhui.,Liu, Yong.,Luo, Sizuo.,Li, Xing.,Yu, Jiaqi.,...&Ding, Dajun.(2019).Coherent interference of molecular electronic states in NO by two-color femtosecond laser pulses.PHYSICAL REVIEW A,99(1),6.
MLA Hu, Wenhui,et al."Coherent interference of molecular electronic states in NO by two-color femtosecond laser pulses".PHYSICAL REVIEW A 99.1(2019):6.
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