DICP OpenIR
Quasi-Amorphous Metallic Nickel Nanopowder as an Efficient and Durable Electrocatalyst for Alkaline Hydrogen Evolution
Zhang, Doudou1,2; Shi, Jingying2; Qi, Yu2; Wang, Xiaomei2; Wang, Hong2; Li, Mingrun2; Liu, Shengzhong1,2; Li, Can2
Corresponding AuthorShi, Jingying(jingyingshi@dicp.ac.cn) ; Liu, Shengzhong(szliu@dicp.ac.cn)
Keywordalkaline solutions chemical synthesis electrocatalysts hydrogen evolution reaction quasi-amorphous metallic nickel
Source PublicationADVANCED SCIENCE
2018-12-01
ISSN2198-3844
DOI10.1002/advs.201801216
Volume5Issue:12Pages:7
Funding ProjectNational Key R&D Program of China[2017YFA0204804] ; National Program on Key Basic Research Project (973 Program)[2014CB239400] ; National Natural Science Foundation of China[21573230] ; Fundamental Research Funds for the Central Universities[2016CBZ002] ; 111 Project[B14041]
Funding OrganizationNational Key R&D Program of China ; National Key R&D Program of China ; National Program on Key Basic Research Project (973 Program) ; National Program on Key Basic Research Project (973 Program) ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; 111 Project ; 111 Project ; National Key R&D Program of China ; National Key R&D Program of China ; National Program on Key Basic Research Project (973 Program) ; National Program on Key Basic Research Project (973 Program) ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; 111 Project ; 111 Project ; National Key R&D Program of China ; National Key R&D Program of China ; National Program on Key Basic Research Project (973 Program) ; National Program on Key Basic Research Project (973 Program) ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; 111 Project ; 111 Project ; National Key R&D Program of China ; National Key R&D Program of China ; National Program on Key Basic Research Project (973 Program) ; National Program on Key Basic Research Project (973 Program) ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; 111 Project ; 111 Project
WOS SubjectChemistry, Multidisciplinary ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary
WOS Research AreaChemistry ; Science & Technology - Other Topics ; Materials Science
WOS KeywordOXYGEN EVOLUTION ; SULFIDE CATALYST ; HIGHLY EFFICIENT ; WATER ; NANOPARTICLES ; REDUCTION ; TUNGSTEN ; GENERATION ; PHOSPHIDE ; GRAPHENE
AbstractNickel is regarded as the best alternative metal electrocatalyst to platinum for hydrogen evolution reaction (HER). Success in developing a quasi-amorphous metallic nickel (QAMN) nanopowder catalyst using a two-step chemical route for efficient and durable HER in alkaline solution is reported. It is found that the QAMN electrocatalyst exhibits essentially zero overpotential at the cathodic onset while delivering 10 mA cm(-2) at an overpotential of only 240 mV; both performances are far better than what was reported previously using prior metallic nickel catalysts. Taking into account increased surface area, further enhanced activity is attributed to the superior intrinsic activity. Meanwhile, the QAMN catalyst shows excellent stability in accelerated and interrupted polarization in alkaline solution for tens of hours. This study provides a new chemical means to prepare amorphous metallic materials for more efficient catalysis.
Language英语
Funding OrganizationNational Key R&D Program of China ; National Key R&D Program of China ; National Program on Key Basic Research Project (973 Program) ; National Program on Key Basic Research Project (973 Program) ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; 111 Project ; 111 Project ; National Key R&D Program of China ; National Key R&D Program of China ; National Program on Key Basic Research Project (973 Program) ; National Program on Key Basic Research Project (973 Program) ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; 111 Project ; 111 Project ; National Key R&D Program of China ; National Key R&D Program of China ; National Program on Key Basic Research Project (973 Program) ; National Program on Key Basic Research Project (973 Program) ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; 111 Project ; 111 Project ; National Key R&D Program of China ; National Key R&D Program of China ; National Program on Key Basic Research Project (973 Program) ; National Program on Key Basic Research Project (973 Program) ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; 111 Project ; 111 Project
WOS IDWOS:000453685900020
PublisherWILEY
Citation statistics
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/166393
Collection中国科学院大连化学物理研究所
Corresponding AuthorShi, Jingying; Liu, Shengzhong
Affiliation1.Shaanxi Normal Univ, Sch Mat Sci & Engn,Key Lab Appl Surface & Colloid, Shaanxi Engn Lab Adv Energy Technol,Minist Educ, Shaanxi Key Lab Adv Energy Devices,Inst Adv Energ, Xian 710119, Shaanxi, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy IChEM, Dalian 116023, Peoples R China
Recommended Citation
GB/T 7714
Zhang, Doudou,Shi, Jingying,Qi, Yu,et al. Quasi-Amorphous Metallic Nickel Nanopowder as an Efficient and Durable Electrocatalyst for Alkaline Hydrogen Evolution[J]. ADVANCED SCIENCE,2018,5(12):7.
APA Zhang, Doudou.,Shi, Jingying.,Qi, Yu.,Wang, Xiaomei.,Wang, Hong.,...&Li, Can.(2018).Quasi-Amorphous Metallic Nickel Nanopowder as an Efficient and Durable Electrocatalyst for Alkaline Hydrogen Evolution.ADVANCED SCIENCE,5(12),7.
MLA Zhang, Doudou,et al."Quasi-Amorphous Metallic Nickel Nanopowder as an Efficient and Durable Electrocatalyst for Alkaline Hydrogen Evolution".ADVANCED SCIENCE 5.12(2018):7.
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