DICP OpenIR
Multi-inch single-crystalline perovskite membrane for high-detectivity flexible photosensors
Liu, Yucheng1,2,3,4,5; Zhang, Yunxia1,2,3,4,5; Yang, Zhou1,2,3,4,5; Ye, Haochen1,2,3,4,5; Feng, Jiangshan1,2,3,4,5; Xu, Zhuo1,2,3,4,5; Zhang, Xu6; Munir, Rahim7; Liu, Jia1,2,3,4,5; Zuo, Ping1,2,3,4,5; Li, Qingxian1,2,3,4,5; Hu, Mingxin1,2,3,4,5; Meng, Lina1,2,3,4,5; Wang, Kang1,2,3,4,5; Smilgies, Detlef-M.8; Zhao, Guangtao1,2,3,4,5; Xu, Hua1,2,3,4,5; Yang, Zupei1,2,3,4,5; Amassian, Aram7; Li, Jiawei9; Zhao, Kui1,2,3,4,5; Liu, Shengzhong (Frank)1,2,3,4,5,6
Corresponding AuthorZhao, Kui(zhaok@snnu.edu.cn) ; Liu, Shengzhong (Frank)(szliu@dicp.ac.cn)
Source PublicationNATURE COMMUNICATIONS
2018-12-13
ISSN2041-1723
DOI10.1038/s41467-018-07440-2
Volume9Pages:11
Funding ProjectNational Key Research and Development Program of China[2017YFA0204800] ; Fundamental Research Funds for the Central Universities[GK201803012] ; National Natural Science Foundation of China[91733301] ; National Natural Science Foundation of China[61604092] ; National Natural Science Foundation of China[61674098] ; 111 Project[B14041] ; Changjiang Scholar and Innovative Research Team[IRT_14R33] ; Natural Science Basic Research Plan in Shaanxi Province of China[2018JM5132]
Funding OrganizationNational Key Research and Development Program of China ; National Key Research and Development Program of China ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; 111 Project ; 111 Project ; Changjiang Scholar and Innovative Research Team ; Changjiang Scholar and Innovative Research Team ; Natural Science Basic Research Plan in Shaanxi Province of China ; Natural Science Basic Research Plan in Shaanxi Province of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; 111 Project ; 111 Project ; Changjiang Scholar and Innovative Research Team ; Changjiang Scholar and Innovative Research Team ; Natural Science Basic Research Plan in Shaanxi Province of China ; Natural Science Basic Research Plan in Shaanxi Province of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; 111 Project ; 111 Project ; Changjiang Scholar and Innovative Research Team ; Changjiang Scholar and Innovative Research Team ; Natural Science Basic Research Plan in Shaanxi Province of China ; Natural Science Basic Research Plan in Shaanxi Province of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; 111 Project ; 111 Project ; Changjiang Scholar and Innovative Research Team ; Changjiang Scholar and Innovative Research Team ; Natural Science Basic Research Plan in Shaanxi Province of China ; Natural Science Basic Research Plan in Shaanxi Province of China
WOS SubjectMultidisciplinary Sciences
WOS Research AreaScience & Technology - Other Topics
WOS KeywordHALIDE PEROVSKITES ; THIN-FILMS ; GROWTH ; PHOTODETECTORS ; FORMAMIDINIUM ; TEMPERATURE ; CSPBBR3 ; WAFERS ; CL ; BR
AbstractSingle crystalline perovskites exhibit high optical absorption, long carrier lifetime, large carrier mobility, low trap-state-density and high defect tolerance. Unfortunately, all single crystalline perovskites attained so far are limited to bulk single crystals and small area wafers. As such, it is impossible to design highly demanded flexible single-crystalline electronics and wearable devices including displays, touch sensing devices, transistors, etc. Herein we report a method of induced peripheral crystallization to prepare large area flexible single-crystalline membrane (SCM) of phenylethylamine lead iodide (C6H5C2H4NH3)(2)PbI4 with area exceeding 2500 mm(2) and thinness as little as 0.6 mu m. The ultrathin flexible SCM exhibits ultralow defect density, superior uniformity and long-term stability. Using the superior ultrathin membrane, a series of flexible photosensors were designed and fabricated to exhibit very high external quantum efficiency of 26530%, responsivity of 98.17 A W-1 and detectivity as much as 1.62 x 10(15) cm Hz(1/2) W-1 (Jones).
Language英语
Funding OrganizationNational Key Research and Development Program of China ; National Key Research and Development Program of China ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; 111 Project ; 111 Project ; Changjiang Scholar and Innovative Research Team ; Changjiang Scholar and Innovative Research Team ; Natural Science Basic Research Plan in Shaanxi Province of China ; Natural Science Basic Research Plan in Shaanxi Province of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; 111 Project ; 111 Project ; Changjiang Scholar and Innovative Research Team ; Changjiang Scholar and Innovative Research Team ; Natural Science Basic Research Plan in Shaanxi Province of China ; Natural Science Basic Research Plan in Shaanxi Province of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; 111 Project ; 111 Project ; Changjiang Scholar and Innovative Research Team ; Changjiang Scholar and Innovative Research Team ; Natural Science Basic Research Plan in Shaanxi Province of China ; Natural Science Basic Research Plan in Shaanxi Province of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; 111 Project ; 111 Project ; Changjiang Scholar and Innovative Research Team ; Changjiang Scholar and Innovative Research Team ; Natural Science Basic Research Plan in Shaanxi Province of China ; Natural Science Basic Research Plan in Shaanxi Province of China
WOS IDWOS:000453057400008
PublisherNATURE PUBLISHING GROUP
Citation statistics
Cited Times:14[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/166443
Collection中国科学院大连化学物理研究所
Corresponding AuthorZhao, Kui; Liu, Shengzhong (Frank)
Affiliation1.Shaanxi Normal Univ, Minist Educ, Key Lab Appl Surface & Colloid Chem, Xian 710119, Shaanxi, Peoples R China
2.Shaanxi Normal Univ, Shaanxi Key Lab Adv Energy Devices, Xian 710119, Shaanxi, Peoples R China
3.Shaanxi Normal Univ, Shaanxi Engn Lab Adv Energy Technol, Xian 710119, Shaanxi, Peoples R China
4.Shaanxi Normal Univ, Inst Adv Energy Mat, Xian 710119, Shaanxi, Peoples R China
5.Shaanxi Normal Univ, Sch Mat Sci & Engn, Xian 710119, Shaanxi, Peoples R China
6.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, iChEM, Dalian 116023, Peoples R China
7.KAUST, Solar & Photovolta Engn Ctr, Div Phys Sci & Engn, Thuwal 239556900, Saudi Arabia
8.Cornell Univ, Cornell High Energy Synchrotron Source, Ithaca, NY 14850 USA
9.Shaanxi Normal Univ, Sch Phys & Informat Technol, Xian 710119, Shaanxi, Peoples R China
Recommended Citation
GB/T 7714
Liu, Yucheng,Zhang, Yunxia,Yang, Zhou,et al. Multi-inch single-crystalline perovskite membrane for high-detectivity flexible photosensors[J]. NATURE COMMUNICATIONS,2018,9:11.
APA Liu, Yucheng.,Zhang, Yunxia.,Yang, Zhou.,Ye, Haochen.,Feng, Jiangshan.,...&Liu, Shengzhong .(2018).Multi-inch single-crystalline perovskite membrane for high-detectivity flexible photosensors.NATURE COMMUNICATIONS,9,11.
MLA Liu, Yucheng,et al."Multi-inch single-crystalline perovskite membrane for high-detectivity flexible photosensors".NATURE COMMUNICATIONS 9(2018):11.
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