DICP OpenIR
Transition metal-nitrogen sites for electrochemical carbon dioxide reduction reaction
Yan, Chengcheng1,2; Lin, Long1,2; Wang, Guoxiong1,3; Bao, Xinhe1,3
Corresponding AuthorWang, Guoxiong(wanggx@dicp.ac.cn) ; Bao, Xinhe(xhbao@dicp.ac.cn)
KeywordElectrochemical carbon dioxide reduction reaction Metal-nitrogen sites Metal-nitrogen containing macrocyclic complexes Metal organic frameworks Zeolitic imidazolate frameworks Carbon material doped with metal-nitrogen sites
Source PublicationCHINESE JOURNAL OF CATALYSIS
2019
ISSN0253-9837
DOI10.1016/S1872-2067(18)63161-4
Volume40Issue:1Pages:23-37
Funding ProjectNational Key R&D Program of China[2017YFA0700102] ; National Natural Science Foundation of China[21573222] ; National Natural Science Foundation of China[91545202] ; Outstanding Youth Talent Project of Dalian[2017RJ03] ; DMTO Project of Dalian Institute of Chemical Physics, CAS[DICP DMTO201702] ; Strategic Priority Research Program of the Chinese Academy of Sciences[XDB17020200] ; Youth Innovation Promotion Association, CAS[2015145]
Funding OrganizationNational Key R&D Program of China ; National Key R&D Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Outstanding Youth Talent Project of Dalian ; Outstanding Youth Talent Project of Dalian ; DMTO Project of Dalian Institute of Chemical Physics, CAS ; DMTO Project of Dalian Institute of Chemical Physics, CAS ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Youth Innovation Promotion Association, CAS ; Youth Innovation Promotion Association, CAS ; National Key R&D Program of China ; National Key R&D Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Outstanding Youth Talent Project of Dalian ; Outstanding Youth Talent Project of Dalian ; DMTO Project of Dalian Institute of Chemical Physics, CAS ; DMTO Project of Dalian Institute of Chemical Physics, CAS ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Youth Innovation Promotion Association, CAS ; Youth Innovation Promotion Association, CAS ; National Key R&D Program of China ; National Key R&D Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Outstanding Youth Talent Project of Dalian ; Outstanding Youth Talent Project of Dalian ; DMTO Project of Dalian Institute of Chemical Physics, CAS ; DMTO Project of Dalian Institute of Chemical Physics, CAS ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Youth Innovation Promotion Association, CAS ; Youth Innovation Promotion Association, CAS ; National Key R&D Program of China ; National Key R&D Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Outstanding Youth Talent Project of Dalian ; Outstanding Youth Talent Project of Dalian ; DMTO Project of Dalian Institute of Chemical Physics, CAS ; DMTO Project of Dalian Institute of Chemical Physics, CAS ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Youth Innovation Promotion Association, CAS ; Youth Innovation Promotion Association, CAS
WOS SubjectChemistry, Applied ; Chemistry, Physical ; Engineering, Chemical
WOS Research AreaChemistry ; Engineering
WOS KeywordGAS-DIFFUSION ELECTRODES ; OXYGEN REDUCTION ; ORGANIC FRAMEWORKS ; CO2 REDUCTION ; ELECTROCATALYTIC REDUCTION ; HIGHLY EFFICIENT ; COBALT-PORPHYRIN ; HETEROGENEOUS CATALYSTS ; POROUS CARBON ; ELECTROREDUCTION
AbstractElectrochemical CO2 reduction reaction (CO2RR) powered by renewable electricity has emerged as the most promising technique for CO2 conversion, making it possible to realize a carbon-neutral cycle. Highly efficient, robust, and cost-effective catalysts are highly demanded for the near-future practical applications of CO2RR. Previous studies on atomically dispersed metal-nitrogen (M-N-x) sites constituted of earth abundant elements with maximum atom-utilization efficiency have demonstrated their performance towards CO2RR. This review summarizes recent advances on a variety of M-N-x sites-containing transition metal-centered macrocyclic complexes, metal organic frameworks, and M-N-x-doped carbon materials for efficient CO2RR, including both experimental and theoretical studies. The roles of metal centers, coordinated ligands, and conductive supports on the intrinsic activity and selectivity, together with the importance of reaction conditions for improved performance are discussed. The mechanisms of CO2RR over these M-N-x-containing materials are presented to provide useful guidance for the rational design of efficient catalysts towards CO2RR. (C) 2019, Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier B.V. All rights reserved.
Language英语
Funding OrganizationNational Key R&D Program of China ; National Key R&D Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Outstanding Youth Talent Project of Dalian ; Outstanding Youth Talent Project of Dalian ; DMTO Project of Dalian Institute of Chemical Physics, CAS ; DMTO Project of Dalian Institute of Chemical Physics, CAS ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Youth Innovation Promotion Association, CAS ; Youth Innovation Promotion Association, CAS ; National Key R&D Program of China ; National Key R&D Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Outstanding Youth Talent Project of Dalian ; Outstanding Youth Talent Project of Dalian ; DMTO Project of Dalian Institute of Chemical Physics, CAS ; DMTO Project of Dalian Institute of Chemical Physics, CAS ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Youth Innovation Promotion Association, CAS ; Youth Innovation Promotion Association, CAS ; National Key R&D Program of China ; National Key R&D Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Outstanding Youth Talent Project of Dalian ; Outstanding Youth Talent Project of Dalian ; DMTO Project of Dalian Institute of Chemical Physics, CAS ; DMTO Project of Dalian Institute of Chemical Physics, CAS ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Youth Innovation Promotion Association, CAS ; Youth Innovation Promotion Association, CAS ; National Key R&D Program of China ; National Key R&D Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Outstanding Youth Talent Project of Dalian ; Outstanding Youth Talent Project of Dalian ; DMTO Project of Dalian Institute of Chemical Physics, CAS ; DMTO Project of Dalian Institute of Chemical Physics, CAS ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Youth Innovation Promotion Association, CAS ; Youth Innovation Promotion Association, CAS
WOS IDWOS:000453646500004
PublisherSCIENCE PRESS
Citation statistics
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/166477
Collection中国科学院大连化学物理研究所
Corresponding AuthorWang, Guoxiong; Bao, Xinhe
Affiliation1.Chinese Acad Sci, Dalian Inst Chem Phys, CAS Ctr Excellence Nanosci, State Key Lab Catalysis, Dalian 116023, Liaoning, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, Dalian 116023, Liaoning, Peoples R China
Recommended Citation
GB/T 7714
Yan, Chengcheng,Lin, Long,Wang, Guoxiong,et al. Transition metal-nitrogen sites for electrochemical carbon dioxide reduction reaction[J]. CHINESE JOURNAL OF CATALYSIS,2019,40(1):23-37.
APA Yan, Chengcheng,Lin, Long,Wang, Guoxiong,&Bao, Xinhe.(2019).Transition metal-nitrogen sites for electrochemical carbon dioxide reduction reaction.CHINESE JOURNAL OF CATALYSIS,40(1),23-37.
MLA Yan, Chengcheng,et al."Transition metal-nitrogen sites for electrochemical carbon dioxide reduction reaction".CHINESE JOURNAL OF CATALYSIS 40.1(2019):23-37.
Files in This Item:
There are no files associated with this item.
Related Services
Recommend this item
Bookmark
Usage statistics
Export to Endnote
Google Scholar
Similar articles in Google Scholar
[Yan, Chengcheng]'s Articles
[Lin, Long]'s Articles
[Wang, Guoxiong]'s Articles
Baidu academic
Similar articles in Baidu academic
[Yan, Chengcheng]'s Articles
[Lin, Long]'s Articles
[Wang, Guoxiong]'s Articles
Bing Scholar
Similar articles in Bing Scholar
[Yan, Chengcheng]'s Articles
[Lin, Long]'s Articles
[Wang, Guoxiong]'s Articles
Terms of Use
No data!
Social Bookmark/Share
All comments (0)
No comment.
 

Items in the repository are protected by copyright, with all rights reserved, unless otherwise indicated.