DICP OpenIR
Graphdiyne as a Host Active Material for Perovskite Solar Cell Application
Li, Jiangsheng1; Jiu, Tonggang1,3,6; Chen, Siqi1; Liu, Le1; Yao, Quantong1; Bi, Fuzhen1; Zhao, Chengjie1; Wang, Zhen1; Zhao, Min1; Zhang, Guodong1; Xue, Yurui2; Lu, Fushen4,5; Li, Yuliang2,3
Corresponding AuthorJiu, Tonggang(jiutg@qibebt.ac.cn) ; Li, Yuliang(ylli@iccas.ac.cn)
KeywordGraphdiyne host active material MAPbI(3) perovskite device solar cells
Source PublicationNANO LETTERS
2018-11-01
ISSN1530-6984
DOI10.1021/acs.nanolett.8b02863
Volume18Issue:11Pages:6941-6947
Funding ProjectMajor Program of Shandong Province Natural Science Foundation[ZR2017ZB0313] ; National Natural Science Foundation of China[51672288] ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; DICP QIBEBT[UN201705] ; Dalian National Laboratory For Clean Energy ; Open Foundation of Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province
Funding OrganizationMajor Program of Shandong Province Natural Science Foundation ; Major Program of Shandong Province Natural Science Foundation ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; DICP QIBEBT ; DICP QIBEBT ; Dalian National Laboratory For Clean Energy ; Dalian National Laboratory For Clean Energy ; Open Foundation of Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province ; Open Foundation of Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province ; Major Program of Shandong Province Natural Science Foundation ; Major Program of Shandong Province Natural Science Foundation ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; DICP QIBEBT ; DICP QIBEBT ; Dalian National Laboratory For Clean Energy ; Dalian National Laboratory For Clean Energy ; Open Foundation of Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province ; Open Foundation of Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province ; Major Program of Shandong Province Natural Science Foundation ; Major Program of Shandong Province Natural Science Foundation ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; DICP QIBEBT ; DICP QIBEBT ; Dalian National Laboratory For Clean Energy ; Dalian National Laboratory For Clean Energy ; Open Foundation of Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province ; Open Foundation of Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province ; Major Program of Shandong Province Natural Science Foundation ; Major Program of Shandong Province Natural Science Foundation ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; DICP QIBEBT ; DICP QIBEBT ; Dalian National Laboratory For Clean Energy ; Dalian National Laboratory For Clean Energy ; Open Foundation of Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province ; Open Foundation of Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province
WOS SubjectChemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
WOS Research AreaChemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
WOS KeywordELECTRON-TRANSPORT ; 2D GRAPHDIYNE ; EFFICIENT ; EXTRACTION
AbstractThis work demonstrates a novel photovoltaic application in which graphdiyne (GD) can be employed as a host material in a perovskite active layer for the first time. In the device fabrication, the best molar ratio for active materials is verified as PbI2/MAI/GD being 1:1:0.25, yielding a peak power-conversion efficiency of 21.01%. We find that graphdiyne, as the host material, exerts significant influence on the crystallization, film morphology, and a series of optoelectronic properties of the perovskite active layer. A uniform MAPbI(3) film with highly crystalline qualities, large domain sizes, and few grain boundaries was realized with the introduction of graphdiyne. Moreover, the current-voltage hysteresis was negligible, and device stability was significantly improved as well. The results indicate that graphdiyne as the host active material presents great potential for the enhancement of the performance of perovskite solar cells.
Language英语
Funding OrganizationMajor Program of Shandong Province Natural Science Foundation ; Major Program of Shandong Province Natural Science Foundation ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; DICP QIBEBT ; DICP QIBEBT ; Dalian National Laboratory For Clean Energy ; Dalian National Laboratory For Clean Energy ; Open Foundation of Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province ; Open Foundation of Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province ; Major Program of Shandong Province Natural Science Foundation ; Major Program of Shandong Province Natural Science Foundation ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; DICP QIBEBT ; DICP QIBEBT ; Dalian National Laboratory For Clean Energy ; Dalian National Laboratory For Clean Energy ; Open Foundation of Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province ; Open Foundation of Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province ; Major Program of Shandong Province Natural Science Foundation ; Major Program of Shandong Province Natural Science Foundation ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; DICP QIBEBT ; DICP QIBEBT ; Dalian National Laboratory For Clean Energy ; Dalian National Laboratory For Clean Energy ; Open Foundation of Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province ; Open Foundation of Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province ; Major Program of Shandong Province Natural Science Foundation ; Major Program of Shandong Province Natural Science Foundation ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; DICP QIBEBT ; DICP QIBEBT ; Dalian National Laboratory For Clean Energy ; Dalian National Laboratory For Clean Energy ; Open Foundation of Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province ; Open Foundation of Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong Province
WOS IDWOS:000451102100038
PublisherAMER CHEMICAL SOC
Citation statistics
Cited Times:7[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/166507
Collection中国科学院大连化学物理研究所
Corresponding AuthorJiu, Tonggang; Li, Yuliang
Affiliation1.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Qingdao 266101, Peoples R China
2.Chinese Acad Sci, Inst Chem, BNLMS, Beijing 100190, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
4.Shantou Univ, Dept Chem, Shantou 515063, Guangdong, Peoples R China
5.Shantou Univ, Key Lab Preparat & Applicat Ordered Struct Mat Gu, Shantou 515063, Guangdong, Peoples R China
6.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
Recommended Citation
GB/T 7714
Li, Jiangsheng,Jiu, Tonggang,Chen, Siqi,et al. Graphdiyne as a Host Active Material for Perovskite Solar Cell Application[J]. NANO LETTERS,2018,18(11):6941-6947.
APA Li, Jiangsheng.,Jiu, Tonggang.,Chen, Siqi.,Liu, Le.,Yao, Quantong.,...&Li, Yuliang.(2018).Graphdiyne as a Host Active Material for Perovskite Solar Cell Application.NANO LETTERS,18(11),6941-6947.
MLA Li, Jiangsheng,et al."Graphdiyne as a Host Active Material for Perovskite Solar Cell Application".NANO LETTERS 18.11(2018):6941-6947.
Files in This Item:
There are no files associated with this item.
Related Services
Recommend this item
Bookmark
Usage statistics
Export to Endnote
Google Scholar
Similar articles in Google Scholar
[Li, Jiangsheng]'s Articles
[Jiu, Tonggang]'s Articles
[Chen, Siqi]'s Articles
Baidu academic
Similar articles in Baidu academic
[Li, Jiangsheng]'s Articles
[Jiu, Tonggang]'s Articles
[Chen, Siqi]'s Articles
Bing Scholar
Similar articles in Bing Scholar
[Li, Jiangsheng]'s Articles
[Jiu, Tonggang]'s Articles
[Chen, Siqi]'s Articles
Terms of Use
No data!
Social Bookmark/Share
All comments (0)
No comment.
 

Items in the repository are protected by copyright, with all rights reserved, unless otherwise indicated.