DICP OpenIR
Visible-Light Driven Overall Conversion of CO2 and H2O to CH4 and O-2 on 3D-SiC@2D-MoS2 Heterostructure
Wang, Ying1,2; Zhang, Zizhong1; Zhang, Lina1; Luo, Zhongbin1; Shen, Jinni1; Lin, Huaxiang1; Long, Jinlin1; Wu, Jeffrey C. S.3; Fu, Xianzhi1; Wang, Xuxu1; Li, Can4
Corresponding AuthorZhang, Zizhong(z.zhang@fzu.edu.cn) ; Wang, Xuxu(xwang@fzu.edu.cn) ; Li, Can(canli@dicp.ac.cn)
Source PublicationJOURNAL OF THE AMERICAN CHEMICAL SOCIETY
2018-11-07
ISSN0002-7863
DOI10.1021/jacs.8b09344
Volume140Issue:44Pages:14595-14598
Funding ProjectNational Natural Science Foundation of China[21673043] ; National Natural Science Foundation of China[21673042] ; National Natural Science Foundation of China[51702053] ; National Natural Science Foundation of China[U1305242]
Funding OrganizationNational Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China
WOS SubjectChemistry, Multidisciplinary
WOS Research AreaChemistry
WOS KeywordPHOTOCATALYTIC H-2 PRODUCTION ; OXYGEN-ISOTOPE EXCHANGE ; CARRIER MOBILITY ; REDUCTION ; OXIDATION ; PHOTOREDUCTION ; PERFORMANCE ; HYDROGEN ; TIO2
AbstractA marigold-like SiC@MoS2 nanoflower with a unique Z-scheme structure efficiently achieves the overall conversion of gas phase CO2 with H2O (CO2 (g) + 2H(2)O (g) = CH4 + 2O(2)) without any sacrificial reagents under visible light (lambda >= 420 nm) irradiation. The CH4 and O-2 evolution are 323 and 621 mu L-g-(1).h(-1), and stable throughout 5 cycle reactions of total 40 h. This work demonstrates a breakthrough in artificial photosynthesis with the Z-scheme 1D heterojunction constructed by combining 2D semiconductor and 3D semiconductor based on the transfer balance of photogenerated electron and hole.
Language英语
Funding OrganizationNational Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China
WOS IDWOS:000449887800015
PublisherAMER CHEMICAL SOC
Citation statistics
Cited Times:22[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/166625
Collection中国科学院大连化学物理研究所
Corresponding AuthorZhang, Zizhong; Wang, Xuxu; Li, Can
Affiliation1.Fuzhou Univ, Coll Chem, State Key Lab Photocatalysis Energy & Environm, Fuzhou 350108, Fujian, Peoples R China
2.Qingdao Univ Sci & Technol, Coll Chem & Mol Engn, Key Lab Inorgan Synthet & Appl Chem, State Key Lab Base Ecochem Engn, Qingdao 266042, Peoples R China
3.Natl Taiwan Univ, Dept Chem Engn, Taipei 10617, Taiwan
4.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
Recommended Citation
GB/T 7714
Wang, Ying,Zhang, Zizhong,Zhang, Lina,et al. Visible-Light Driven Overall Conversion of CO2 and H2O to CH4 and O-2 on 3D-SiC@2D-MoS2 Heterostructure[J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,2018,140(44):14595-14598.
APA Wang, Ying.,Zhang, Zizhong.,Zhang, Lina.,Luo, Zhongbin.,Shen, Jinni.,...&Li, Can.(2018).Visible-Light Driven Overall Conversion of CO2 and H2O to CH4 and O-2 on 3D-SiC@2D-MoS2 Heterostructure.JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,140(44),14595-14598.
MLA Wang, Ying,et al."Visible-Light Driven Overall Conversion of CO2 and H2O to CH4 and O-2 on 3D-SiC@2D-MoS2 Heterostructure".JOURNAL OF THE AMERICAN CHEMICAL SOCIETY 140.44(2018):14595-14598.
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