DICP OpenIR
Gas-solid reaction based over one-micrometer thick stable perovskite films for efficient solar cells and modules
Liu, Zonghao1; Qiu, Longbin1; Juarez-Perez, Emilio J.1; Hawash, Zafer1; Kim, Taehoon1; Jiang, Yan1; Wu, Zhifang1; Raga, Sonia R.1; Ono, Luis K.1; Liu, Shengzhong (Frank)2,3; Qi, Yabing1
Corresponding AuthorQi, Yabing(Yabing.Qi@OIST.jp)
Source PublicationNATURE COMMUNICATIONS
2018-09-24
ISSN2041-1723
DOI10.1038/s41467-018-06317-8
Volume9Pages:11
Funding ProjectEnergy Materials and Surface Sciences Unit of the Okinawa Institute of Science and Technology Graduate University ; OIST Proof of Concept (POC) Program ; OIST R&D Cluster Research Program ; JSPS KAKENHI Grant[JP18K05266] ; 111 Project[B14041]
Funding OrganizationEnergy Materials and Surface Sciences Unit of the Okinawa Institute of Science and Technology Graduate University ; Energy Materials and Surface Sciences Unit of the Okinawa Institute of Science and Technology Graduate University ; OIST Proof of Concept (POC) Program ; OIST Proof of Concept (POC) Program ; OIST R&D Cluster Research Program ; OIST R&D Cluster Research Program ; JSPS KAKENHI Grant ; JSPS KAKENHI Grant ; 111 Project ; 111 Project ; Energy Materials and Surface Sciences Unit of the Okinawa Institute of Science and Technology Graduate University ; Energy Materials and Surface Sciences Unit of the Okinawa Institute of Science and Technology Graduate University ; OIST Proof of Concept (POC) Program ; OIST Proof of Concept (POC) Program ; OIST R&D Cluster Research Program ; OIST R&D Cluster Research Program ; JSPS KAKENHI Grant ; JSPS KAKENHI Grant ; 111 Project ; 111 Project ; Energy Materials and Surface Sciences Unit of the Okinawa Institute of Science and Technology Graduate University ; Energy Materials and Surface Sciences Unit of the Okinawa Institute of Science and Technology Graduate University ; OIST Proof of Concept (POC) Program ; OIST Proof of Concept (POC) Program ; OIST R&D Cluster Research Program ; OIST R&D Cluster Research Program ; JSPS KAKENHI Grant ; JSPS KAKENHI Grant ; 111 Project ; 111 Project ; Energy Materials and Surface Sciences Unit of the Okinawa Institute of Science and Technology Graduate University ; Energy Materials and Surface Sciences Unit of the Okinawa Institute of Science and Technology Graduate University ; OIST Proof of Concept (POC) Program ; OIST Proof of Concept (POC) Program ; OIST R&D Cluster Research Program ; OIST R&D Cluster Research Program ; JSPS KAKENHI Grant ; JSPS KAKENHI Grant ; 111 Project ; 111 Project
WOS SubjectMultidisciplinary Sciences
WOS Research AreaScience & Technology - Other Topics
WOS KeywordORGANOMETAL TRIHALIDE PEROVSKITE ; INORGANIC HALIDE PEROVSKITES ; METHYLAMINE-GAS ; SINGLE-CRYSTALS ; CH3NH3PBI3 ; STABILITY ; LIGHT ; INTERFACE ; TRANSPORT ; EVOLUTION
AbstractBesides high efficiency, the stability and reproducibility of perovskite solar cells (PSCs) are also key for their commercialization. Herein, we report a simple perovskite formation method to fabricate perovskite films with thickness over 1 mu m in ambient condition on the basis of the fast gas-solid reaction of chlorine-incorporated hydrogen lead triiodide and methylamine gas. The resultant thick and smooth chlorine-incorporated perovskite films exhibit full coverage, improved crystallinity, low surface roughness and low thickness variation. The resultant PSCs achieve an average power conversion efficiency of 19.1 +/- 0.4% with good reproducibility. Meanwhile, this method enables an active area efficiency of 15.3% for 5 cmx 5 cm solar modules. The un-encapsulated PSCs exhibit an excellent T-80 lifetime exceeding 1600 h under continuous operation conditions in dry nitrogen environment.
Language英语
Funding OrganizationEnergy Materials and Surface Sciences Unit of the Okinawa Institute of Science and Technology Graduate University ; Energy Materials and Surface Sciences Unit of the Okinawa Institute of Science and Technology Graduate University ; OIST Proof of Concept (POC) Program ; OIST Proof of Concept (POC) Program ; OIST R&D Cluster Research Program ; OIST R&D Cluster Research Program ; JSPS KAKENHI Grant ; JSPS KAKENHI Grant ; 111 Project ; 111 Project ; Energy Materials and Surface Sciences Unit of the Okinawa Institute of Science and Technology Graduate University ; Energy Materials and Surface Sciences Unit of the Okinawa Institute of Science and Technology Graduate University ; OIST Proof of Concept (POC) Program ; OIST Proof of Concept (POC) Program ; OIST R&D Cluster Research Program ; OIST R&D Cluster Research Program ; JSPS KAKENHI Grant ; JSPS KAKENHI Grant ; 111 Project ; 111 Project ; Energy Materials and Surface Sciences Unit of the Okinawa Institute of Science and Technology Graduate University ; Energy Materials and Surface Sciences Unit of the Okinawa Institute of Science and Technology Graduate University ; OIST Proof of Concept (POC) Program ; OIST Proof of Concept (POC) Program ; OIST R&D Cluster Research Program ; OIST R&D Cluster Research Program ; JSPS KAKENHI Grant ; JSPS KAKENHI Grant ; 111 Project ; 111 Project ; Energy Materials and Surface Sciences Unit of the Okinawa Institute of Science and Technology Graduate University ; Energy Materials and Surface Sciences Unit of the Okinawa Institute of Science and Technology Graduate University ; OIST Proof of Concept (POC) Program ; OIST Proof of Concept (POC) Program ; OIST R&D Cluster Research Program ; OIST R&D Cluster Research Program ; JSPS KAKENHI Grant ; JSPS KAKENHI Grant ; 111 Project ; 111 Project
WOS IDWOS:000445329000015
PublisherNATURE PUBLISHING GROUP
Citation statistics
Cited Times:5[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/167011
Collection中国科学院大连化学物理研究所
Corresponding AuthorQi, Yabing
Affiliation1.Grad Univ, OIST, EMSSU, 1919-1 Tancha, Okinawa 9040495, Japan
2.Shaanxi Normal Univ, Key Lab Appl Surface & Colloid Chem, Shaanxi Key Lab Adv Energy Devices,Sch Mat Sci &, Shaanxi Engn Lab Adv Energy Technol,Minist Educ, Xian 710119, Shaanxi, Peoples R China
3.Chinese Acad Sci, Dalian Inst Chem Phys, iChEM, Dalian Natl Lab Clean Energy, 457 Zhongshan Rd, Dalian 116023, Peoples R China
Recommended Citation
GB/T 7714
Liu, Zonghao,Qiu, Longbin,Juarez-Perez, Emilio J.,et al. Gas-solid reaction based over one-micrometer thick stable perovskite films for efficient solar cells and modules[J]. NATURE COMMUNICATIONS,2018,9:11.
APA Liu, Zonghao.,Qiu, Longbin.,Juarez-Perez, Emilio J..,Hawash, Zafer.,Kim, Taehoon.,...&Qi, Yabing.(2018).Gas-solid reaction based over one-micrometer thick stable perovskite films for efficient solar cells and modules.NATURE COMMUNICATIONS,9,11.
MLA Liu, Zonghao,et al."Gas-solid reaction based over one-micrometer thick stable perovskite films for efficient solar cells and modules".NATURE COMMUNICATIONS 9(2018):11.
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