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Regio- and Diastereoselective Access to Fused Isoxazolidines via Ru(II)-Catalyzed C-H Activation of Nitrones and Coupling with Perfluoroalkylolefins
Li, Yunyun1,2; Xie, Fang1; Liu, Yuan1; Yang, Xifa1,2; Li, Xingwei1
Source PublicationORGANIC LETTERS
2018-01-19
ISSN1523-7060
DOI10.1021/acs.orglett.7b03775
Volume20Issue:2Pages:437-440
Indexed BySCI
SubtypeArticle
WOS HeadingsScience & Technology ; Physical Sciences
WOS SubjectChemistry, Organic
WOS Research AreaChemistry
WOS Keyword1,3-DIPOLAR CYCLOADDITION REACTIONS ; ENANTIOSELECTIVE FLUORINATION ; AZOMETHINE YLIDES ; ORGANIC-SYNTHESIS ; ROOM-TEMPERATURE ; DIRECTING GROUPS ; ZETEKITOXIN-AB ; FUNCTIONALIZATION ; FLUOROALKENYLATION ; PALLADIUM
AbstractThe synthsis of fluorinated isoxazolidines in bicyclic settings has been realized via Ru(II)-catalyzed C-H activation of aryl nitrones with perfluoroalkyl-substituted olefins as the coupling partner. The reaction proceeded via initial chelation-assisted C(aryl)-H allylation followed by regio- and diastereoselective intramolecular dipolar addition between the nitrone directing group and the olefin unit.
Language英语
WOS IDWOS:000423252400031
PublisherAMER CHEMICAL SOC
Citation statistics
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/168611
Collection中国科学院大连化学物理研究所
Corresponding AuthorLi, Xingwei
Affiliation1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
Recommended Citation
GB/T 7714
Li, Yunyun,Xie, Fang,Liu, Yuan,et al. Regio- and Diastereoselective Access to Fused Isoxazolidines via Ru(II)-Catalyzed C-H Activation of Nitrones and Coupling with Perfluoroalkylolefins[J]. ORGANIC LETTERS,2018,20(2):437-440.
APA Li, Yunyun,Xie, Fang,Liu, Yuan,Yang, Xifa,&Li, Xingwei.(2018).Regio- and Diastereoselective Access to Fused Isoxazolidines via Ru(II)-Catalyzed C-H Activation of Nitrones and Coupling with Perfluoroalkylolefins.ORGANIC LETTERS,20(2),437-440.
MLA Li, Yunyun,et al."Regio- and Diastereoselective Access to Fused Isoxazolidines via Ru(II)-Catalyzed C-H Activation of Nitrones and Coupling with Perfluoroalkylolefins".ORGANIC LETTERS 20.2(2018):437-440.
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