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Engineering Fractal MTW Zeolite Mesocrystal: Particle-Based Dendritic Growth via Twinning-Plane Induced Crystallization
Zhao, Yang1,2; Ye, Zhaoqi1,2; Wang, Lei1,2,6; Zhang, Hongbin3; Xue, Fangqi1,2; Xie, Songhai1,2; Cao, Xiao-Ming4,5; Zhang, Yahong1,2; Tang, Yi1,2
Source PublicationCRYSTAL GROWTH & DESIGN
2018-02-01
ISSN1528-7483
DOI10.1021/acs.cgd.7b01547
Volume18Issue:2Pages:1101-1108
Indexed BySCI
SubtypeArticle
WOS HeadingsScience & Technology ; Physical Sciences ; Technology
WOS SubjectChemistry, Multidisciplinary ; Crystallography ; Materials Science, Multidisciplinary
WOS Research AreaChemistry ; Crystallography ; Materials Science
WOS KeywordHETEROGENEOUS SYSTEM ; ORIENTED ATTACHMENT ; ZSM-12 ZEOLITE ; MECHANISM ; MORPHOLOGY ; TEMPLATES ; EVOLUTION ; DIRECTION ; PATHWAYS ; CRYSTALS
AbstractConstructing superstructured crystalline :materials by crystal engineering is an attractive objective for miscellaneous fields of researchers spanning biominietics to catalytic materials. Zeolite is a kind of important crystalline catalyst, and superstructured zeolite has great potential for wideSpread applications. However, the ambiguous crystallization mechanisms hamper the effective and scientific fabrication of superstructured zeolite with exceptional properties. Herein, a fractal superstructured MTW zeolite with mesocrystal side branches is prepared via, a nanoparticle-based nonclassical pathway with twinning plane induced crystallization, which is distinct from the formation of general mesocrystal via crystal-crystal oriented attachment. Deformed atomic connection at a specific crystallographic plane contributes to the production of side branches. Moreover, this intriguing morphology could be regulated merely via adjusting the crystallization kinetics based on the unequivocal nonclassical crystallization mechanism. It will open a new avenue for design and synthesis of targeted crystals with superstructure and extraordinary properties.
Language英语
WOS IDWOS:000424851400066
PublisherAMER CHEMICAL SOC
Citation statistics
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/168831
Collection中国科学院大连化学物理研究所
Corresponding AuthorZhang, Hongbin; Tang, Yi
Affiliation1.Fudan Univ, Collaborat Innovat Ctr Chem Energy Mat, Dept Chem, Lab Adv Mat, Shanghai 200433, Peoples R China
2.Fudan Univ, Shanghai Key Lab Mol Catalysis & Innovat Mat, Shanghai 200433, Peoples R China
3.Fudan Univ Lib, Inst Preservat Chinese Ancient Books, Shanghai 200433, Peoples R China
4.East China Univ Sci & Technol, Ctr Computat Chem, Key Lab Adv Mat, Shanghai 200237, Peoples R China
5.East China Univ Sci & Technol, Sch Chem & Mol Engn, Res Inst Ind Catalysis, Shanghai 200237, Peoples R China
6.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian, Peoples R China
Recommended Citation
GB/T 7714
Zhao, Yang,Ye, Zhaoqi,Wang, Lei,et al. Engineering Fractal MTW Zeolite Mesocrystal: Particle-Based Dendritic Growth via Twinning-Plane Induced Crystallization[J]. CRYSTAL GROWTH & DESIGN,2018,18(2):1101-1108.
APA Zhao, Yang.,Ye, Zhaoqi.,Wang, Lei.,Zhang, Hongbin.,Xue, Fangqi.,...&Tang, Yi.(2018).Engineering Fractal MTW Zeolite Mesocrystal: Particle-Based Dendritic Growth via Twinning-Plane Induced Crystallization.CRYSTAL GROWTH & DESIGN,18(2),1101-1108.
MLA Zhao, Yang,et al."Engineering Fractal MTW Zeolite Mesocrystal: Particle-Based Dendritic Growth via Twinning-Plane Induced Crystallization".CRYSTAL GROWTH & DESIGN 18.2(2018):1101-1108.
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