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Modulating the CO methanation activity of Ni catalyst by nitrogen doped carbon
Lin, Yaping1,2; Li, Pan1; Cui, Tingting1,2; Pan, Xiulian1; Bao, Xinhe1
KeywordCo Methanation Ni Catalyst Carbon Nitrogen Doping Sic
Source PublicationJOURNAL OF ENERGY CHEMISTRY
2018-05-01
ISSN2095-4956
DOI10.1016/j.jechem.2017.06.008
Volume27Issue:3Pages:898-902
Indexed BySCI
SubtypeArticle
WOS HeadingsScience & Technology ; Physical Sciences ; Technology
WOS SubjectChemistry, Applied ; Chemistry, Physical ; Energy & Fuels ; Engineering, Chemical
WOS Research AreaChemistry ; Energy & Fuels ; Engineering
WOS KeywordFISCHER-TROPSCH SYNTHESIS ; SYNTHETIC NATURAL-GAS ; OXYGEN REDUCTION ; IRON CATALYSTS ; GRAPHENE ; PERFORMANCE ; 1ST-PRINCIPLE ; HYDROGENATION ; NANOTUBES ; NI(111)
AbstractNitrogen doping has been proved to be an effective way to modify the properties of graphene and other carbon materials. Herein, we explore a composite with nitrogen doped carbon overlayers wrapping SiC substrate as a support for Ni (Ni/CN-SiC) and evaluate its effects on the methanation activity. The results show that both the activity and stability of Ni are enhanced. Characterization with STEM, XRD, XPS, Raman and H-2 - TPR indicates that nitrogen doping generates more defects in the carbon overlayers, which benefit the dispersion of Ni. Furthermore, the reduction of Ni is facilitated. (C) 2017 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier B.V. and Science Press. All rights reserved.
Language英语
WOS IDWOS:000430515900032
PublisherELSEVIER SCIENCE BV
Citation statistics
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/169143
Collection中国科学院大连化学物理研究所
Corresponding AuthorPan, Xiulian; Bao, Xinhe
Affiliation1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Liaoning, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
Recommended Citation
GB/T 7714
Lin, Yaping,Li, Pan,Cui, Tingting,et al. Modulating the CO methanation activity of Ni catalyst by nitrogen doped carbon[J]. JOURNAL OF ENERGY CHEMISTRY,2018,27(3):898-902.
APA Lin, Yaping,Li, Pan,Cui, Tingting,Pan, Xiulian,&Bao, Xinhe.(2018).Modulating the CO methanation activity of Ni catalyst by nitrogen doped carbon.JOURNAL OF ENERGY CHEMISTRY,27(3),898-902.
MLA Lin, Yaping,et al."Modulating the CO methanation activity of Ni catalyst by nitrogen doped carbon".JOURNAL OF ENERGY CHEMISTRY 27.3(2018):898-902.
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