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Chemically Cross-Linked MOF Membrane Generated from Imidazolium-Based Ionic Liquid-Decorated UiO-66 Type NMOF and Its Application toward CO2 Separation and Conversion
Yao, Bing-Jian1; Ding, Luo-Gang1; Li, Fei1; Li, Jiang-Tao1; Fu, Qi-Juan1; Ban, Yujie2; Guo, Ang2; Dong, Yu-Bin1
KeywordMofs Gas Separation Cross-linked Membrane Catalytic Cycloaddition Polyurethane Ionic Liquid
Source PublicationACS APPLIED MATERIALS & INTERFACES
2017-11-08
ISSN1944-8244
DOI10.1021/acsami.7b12697
Volume9Issue:44Pages:38919-38930
Indexed BySCI
SubtypeArticle
WOS HeadingsScience & Technology ; Technology
WOS SubjectNanoscience & Nanotechnology ; Materials Science, Multidisciplinary
WOS Research AreaScience & Technology - Other Topics ; Materials Science
WOS KeywordMIXED-MATRIX MEMBRANES ; METAL-ORGANIC FRAMEWORK ; CARBON-DIOXIDE CAPTURE ; CO2/CH4 SEPARATION ; GAS SEPARATION ; THIN-FILMS ; POLYIMIDE ; CYCLOADDITION ; ADSORPTION ; FUNCTIONALIZATION
AbstractCarbon dioxide capture and transformation are of great importance to make cuts in greenhouse gas emissions. Nanometal-organic frameworks (NMOFs) could serve as ideal fillers for polymer membranes owing to their structural diversity and regulable micro-environment of the nanocage. Herein, a bifunctional, robust, and chemically cross-linked NMOF-based membrane was successfully constructed by the postsynthetic polymerization of imidazolium-based ionic liquid (IL)-decorated UiO-66 type nanoparticles (NPs) and the isocyanate-terminated polyurethane oligomer under mild conditions. The IL-modified MOF-polymer membranes exhibit a highly selective adsorption for CO2 over N-2 and CH4. In addition, the obtained membrane can also be a highly active heterogeneous catalyst for CO2 transformation by cycloaddition with epoxide under an ambient pressure.
Language英语
WOS IDWOS:000415140800081
PublisherAMER CHEMICAL SOC
Citation statistics
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/169251
Collection中国科学院大连化学物理研究所
Corresponding AuthorYao, Bing-Jian; Dong, Yu-Bin
Affiliation1.Shandong Normal Univ, Collaborat Innovat Ctr Functionalized Probes Chem, Coll Chem Chem Engn & Mat Sci, Key Lab Mol & Nano Probes,Minist Educ, Jinan 250014, Shandong, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, 457 Zhongshan Rd, Dalian 116023, Peoples R China
Recommended Citation
GB/T 7714
Yao, Bing-Jian,Ding, Luo-Gang,Li, Fei,et al. Chemically Cross-Linked MOF Membrane Generated from Imidazolium-Based Ionic Liquid-Decorated UiO-66 Type NMOF and Its Application toward CO2 Separation and Conversion[J]. ACS APPLIED MATERIALS & INTERFACES,2017,9(44):38919-38930.
APA Yao, Bing-Jian.,Ding, Luo-Gang.,Li, Fei.,Li, Jiang-Tao.,Fu, Qi-Juan.,...&Dong, Yu-Bin.(2017).Chemically Cross-Linked MOF Membrane Generated from Imidazolium-Based Ionic Liquid-Decorated UiO-66 Type NMOF and Its Application toward CO2 Separation and Conversion.ACS APPLIED MATERIALS & INTERFACES,9(44),38919-38930.
MLA Yao, Bing-Jian,et al."Chemically Cross-Linked MOF Membrane Generated from Imidazolium-Based Ionic Liquid-Decorated UiO-66 Type NMOF and Its Application toward CO2 Separation and Conversion".ACS APPLIED MATERIALS & INTERFACES 9.44(2017):38919-38930.
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