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Recent Advances in Photoelectrochemical Applications of Silicon Materials for Solar-to-Chemicals Conversion
Zhang, Doudou1,2; Shi, Jingying2; Zi, Wei1; Wang, Pengpeng2,3; Liu, Shengzhong (Frank)1,2
KeywordElectrochemistry Photochemistry Semiconductors Silicon Solar-to-chemicals Conversion
Source PublicationCHEMSUSCHEM
2017-11-23
ISSN1864-5631
DOI10.1002/cssc.201701674
Volume10Issue:22Pages:4324-4341
Indexed BySCI
SubtypeReview
WOS HeadingsScience & Technology ; Physical Sciences
WOS SubjectChemistry, Multidisciplinary ; GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY
WOS Research AreaChemistry ; Science & Technology - Other Topics
WOS KeywordTANTALUM NITRIDE PHOTOANODE ; HYDROGEN EVOLUTION REACTION ; EFFICIENT WATER OXIDATION ; LIGHT-INDUCED DEGRADATION ; ATOMIC-LAYER DEPOSITION ; REDOX FLOW BATTERY ; HOLE-STORAGE-LAYER ; AMORPHOUS-SILICON ; MICROCRYSTALLINE SILICON ; ENERGY-CONVERSION
AbstractPhotoelectrochemical (PEC) technology for the conversion of solar energy into chemicals requires cost-effective photoelectrodes to efficiently and stably drive anodic and/or cathodic half-reactions to complete the overall reactions for storing solar energy in chemical bonds. The shared properties among semiconducting photoelectrodes and photovoltaic (PV) materials are light absorption, charge separation, and charge transfer. Earth-abundant silicon materials have been widely applied in the PV industry, and have demonstrated their efficiency as alternative photoabsorbers for photoelectrodes. Many efforts have been made to fabricate silicon photoelectrodes with enhanced performance, and significant progress has been achieved in recent years. Herein, recent developments in crystalline and thin-film silicon-based photoelectrodes (including amorphous, microcrystalline, and nanocrystalline silicon) immersed in aqueous solution for PEC hydrogen production from water splitting are summarized, as well as applications in PEC CO2 reduction and PEC regeneration of discharged species in redox flow batteries. Silicon is an ideal material for the cost-effective production of solar chemicals through PEC methods.
Language英语
WOS IDWOS:000416158500006
PublisherWILEY-V C H VERLAG GMBH
Citation statistics
Cited Times:19[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/169261
Collection中国科学院大连化学物理研究所
Corresponding AuthorShi, Jingying
Affiliation1.Shaanxi Normal Univ, Key Lab Appl Surface & Colloid Chem, Natl Minist Educ,Inst Adv Energy Mat,Sch Mat Sci, Shaanxi Key Lab Adv Energy Devices,Shaanxi Engn L, Xian 710119, Shaanxi, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, State Key Lab Catalysis, Dalian 116023, Liaoning, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
Recommended Citation
GB/T 7714
Zhang, Doudou,Shi, Jingying,Zi, Wei,et al. Recent Advances in Photoelectrochemical Applications of Silicon Materials for Solar-to-Chemicals Conversion[J]. CHEMSUSCHEM,2017,10(22):4324-4341.
APA Zhang, Doudou,Shi, Jingying,Zi, Wei,Wang, Pengpeng,&Liu, Shengzhong .(2017).Recent Advances in Photoelectrochemical Applications of Silicon Materials for Solar-to-Chemicals Conversion.CHEMSUSCHEM,10(22),4324-4341.
MLA Zhang, Doudou,et al."Recent Advances in Photoelectrochemical Applications of Silicon Materials for Solar-to-Chemicals Conversion".CHEMSUSCHEM 10.22(2017):4324-4341.
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