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A shaped binderless ZSM-11 zeolite catalyst for direct amination of isobutene to tert-butylamine
Zhang, Wanshuo1,2; Gao, Shangyao2,3; Xie, Sujuan; Liu, Hui2,4; Zhu, Xiangxue2; Shang, Yongchen1; Liu, Shenglin2; Xu, Longya2; Zhang, Ye5
KeywordBinderless Zeolite Zsm-11 Amination Isobutene Tert-butylamine
Source PublicationCHINESE JOURNAL OF CATALYSIS
2017
ISSN0253-9837
DOI10.1016/S1872-2067(17)62756-6
Volume38Issue:1Pages:168-175
Indexed BySCI
SubtypeArticle
WOS HeadingsScience & Technology ; Physical Sciences ; Technology
WOS SubjectChemistry, Applied ; Chemistry, Physical ; Engineering, Chemical
WOS Research AreaChemistry ; Engineering
WOS KeywordDIMETHYL ETHER ; METHANOL ; PERFORMANCE ; MORDENITE ; BENZENE ; SYSTEMS
AbstractA shaped binderless and two binder-containing ZSM-11 zeolite catalysts were prepared and characterized by powder X-ray diffraction,N-2 adsorption-desorption, and pyridine adsorption-infrared measurements. The binderless catalyst was synthesized using a dry-gel conversion technique, in which 1,6-hexanediamine and tetrabutylammonium bromide were used as structure-directing agents and no other alkaline materials were added. The catalytic performance of the zeolites in the direct amination of isobutene to tert-butylamine was evaluated in a fixed-bed reactor. By virtue of its high crystallinity as well as its good mechanical strength, the shaped binderless ZSM-11 catalyst showed a higher rate of formation of tert-butylamine than did the binder-containing catalysts. (C) 2017, Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier B.V. All rights reserved.
Language英语
WOS IDWOS:000394481400020
PublisherSCIENCE PRESS
Citation statistics
Cited Times:8[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/169509
Collection中国科学院大连化学物理研究所
Corresponding AuthorShang, Yongchen; Liu, Shenglin
Affiliation1.Harbin Normal Univ, Coll Chem & Chem Engn, Harbin 150025, Heilongjiang, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Liaoning, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
4.Sinochem Quanzhou Petrochem Co Ltd, Ctr Res & Dev, Quanzhou 362103, Fujian, Peoples R China
5.PetroChina Fushun Petrochem Co, Fushun 113008, Liaoning, Peoples R China
Recommended Citation
GB/T 7714
Zhang, Wanshuo,Gao, Shangyao,Xie, Sujuan,et al. A shaped binderless ZSM-11 zeolite catalyst for direct amination of isobutene to tert-butylamine[J]. CHINESE JOURNAL OF CATALYSIS,2017,38(1):168-175.
APA Zhang, Wanshuo.,Gao, Shangyao.,Xie, Sujuan.,Liu, Hui.,Zhu, Xiangxue.,...&Zhang, Ye.(2017).A shaped binderless ZSM-11 zeolite catalyst for direct amination of isobutene to tert-butylamine.CHINESE JOURNAL OF CATALYSIS,38(1),168-175.
MLA Zhang, Wanshuo,et al."A shaped binderless ZSM-11 zeolite catalyst for direct amination of isobutene to tert-butylamine".CHINESE JOURNAL OF CATALYSIS 38.1(2017):168-175.
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