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A facile strategy to fabricate carboxyl-rich carbon spheres with copper-based MOFs through coordination bond
Ge, Chunhua1; Du, Yan1; Wang, Rui1; Xue, Lili1; Wu, Zhongshuai2; Xing, Tianzhu1; Ji, Xiaochun1; Ma, Lin1; Zhang, Xiangdong1
KeywordCarbon Spheres Mofs Composites Catalysis
Source PublicationJOURNAL OF POROUS MATERIALS
2016-12-01
ISSN1380-2224
DOI10.1007/s10934-016-0214-z
Volume23Issue:6Pages:1537-1545
Indexed BySCI
SubtypeArticle
WOS HeadingsScience & Technology ; Physical Sciences ; Technology
WOS SubjectChemistry, Applied ; Chemistry, Physical ; Materials Science, Multidisciplinary
WOS Research AreaChemistry ; Materials Science
WOS KeywordMETAL-ORGANIC FRAMEWORKS ; OXIDE COMPOSITES ; CORE-SHELL ; BENZYL ALCOHOL ; ADSORPTION ; OXIDATION ; MICROSPHERES ; CATALYST ; AMMONIA ; STORAGE
AbstractA new composite (CCSs/MOFs) of carboxyl-rich carbon spheres (CCSs) and copper-based metal-organic frameworks (MOFs) was for the first time prepared. The CCSs/MOFs composite was synthesized by the coordinated growth of high surface area and porous MOFs, [Cu-3(BTC)(2)(H2O)](n) (HKUST-1), on the surface of the functionalized CCSs obtained through a one-step hydrothermal carbonization of glucose with acrylic acid at 180 A degrees C for 24 h. The resulting composites showed a core/shell structure with a tunable diameter arranging from 0.6 to 3.0 mu m, and possessed high specific surface area of 495 m(2)/g and nanoporous structures derived from MOFs. Further, the catalytic oxidation of benzylic alcohol to benzaldehyde as its application was studied.
Language英语
WOS IDWOS:000387111500014
PublisherSPRINGER
Citation statistics
Cited Times:3[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/169819
Collection中国科学院大连化学物理研究所
Corresponding AuthorZhang, Xiangdong
Affiliation1.Liaoning Univ, Coll Chem, Shenyang 110036, Liaoning, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, Dalian 116023, Peoples R China
Recommended Citation
GB/T 7714
Ge, Chunhua,Du, Yan,Wang, Rui,et al. A facile strategy to fabricate carboxyl-rich carbon spheres with copper-based MOFs through coordination bond[J]. JOURNAL OF POROUS MATERIALS,2016,23(6):1537-1545.
APA Ge, Chunhua.,Du, Yan.,Wang, Rui.,Xue, Lili.,Wu, Zhongshuai.,...&Zhang, Xiangdong.(2016).A facile strategy to fabricate carboxyl-rich carbon spheres with copper-based MOFs through coordination bond.JOURNAL OF POROUS MATERIALS,23(6),1537-1545.
MLA Ge, Chunhua,et al."A facile strategy to fabricate carboxyl-rich carbon spheres with copper-based MOFs through coordination bond".JOURNAL OF POROUS MATERIALS 23.6(2016):1537-1545.
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