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Manganese(I)-Catalyzed Synthesis of Fused Eight- and Four-Membered Carbocycles via C-H Activation and Pericyclic Reactions
Xu, Youwei1,3; Zheng, Guangfan2; Kong, Lingheng2; Li, Xingwei1,2
Corresponding AuthorLi, Xingwei(xwli@dicp.ac.cn)
Source PublicationORGANIC LETTERS
2019-05-03
ISSN1523-7060
DOI10.1021/acs.orglett.9b01139
Volume21Issue:9Pages:3402-3406
Funding ProjectDalian Institute of Chemical Physics (Chinese Academy of Sciences) ; NSFC[21525208] ; NSFC[21472186]
Funding OrganizationDalian Institute of Chemical Physics (Chinese Academy of Sciences) ; Dalian Institute of Chemical Physics (Chinese Academy of Sciences) ; NSFC ; NSFC ; Dalian Institute of Chemical Physics (Chinese Academy of Sciences) ; Dalian Institute of Chemical Physics (Chinese Academy of Sciences) ; NSFC ; NSFC ; Dalian Institute of Chemical Physics (Chinese Academy of Sciences) ; Dalian Institute of Chemical Physics (Chinese Academy of Sciences) ; NSFC ; NSFC ; Dalian Institute of Chemical Physics (Chinese Academy of Sciences) ; Dalian Institute of Chemical Physics (Chinese Academy of Sciences) ; NSFC ; NSFC
WOS SubjectChemistry, Organic
WOS Research AreaChemistry
WOS Keyword2+2 CYCLOADDITIONS ; DIRECTING GROUPS ; N BOND ; ALLENES ; FUNCTIONALIZATIONS ; ALLYLATION ; ALKYNES ; ARENES ; COMBINATION ; CYCLIZATION
AbstractPericyclic reactions have allowed facile construction of complex cycles. On the other hand, metal-catalyzed C-H activation has been established as an important strategy for rapid synthesis of complex structures. The two areas are integrated in Mn(I)-catalyzed redox-neutral coupling of 3-alkenyl- and 3-allylindoles with propargylic carbonates, which occurred via C-H allenylation with subsequent pericyclic reactions to afford fused eight- and four-membered carbocycles, respectively.
Language英语
Funding OrganizationDalian Institute of Chemical Physics (Chinese Academy of Sciences) ; Dalian Institute of Chemical Physics (Chinese Academy of Sciences) ; NSFC ; NSFC ; Dalian Institute of Chemical Physics (Chinese Academy of Sciences) ; Dalian Institute of Chemical Physics (Chinese Academy of Sciences) ; NSFC ; NSFC ; Dalian Institute of Chemical Physics (Chinese Academy of Sciences) ; Dalian Institute of Chemical Physics (Chinese Academy of Sciences) ; NSFC ; NSFC ; Dalian Institute of Chemical Physics (Chinese Academy of Sciences) ; Dalian Institute of Chemical Physics (Chinese Academy of Sciences) ; NSFC ; NSFC
WOS IDWOS:000467320000090
PublisherAMER CHEMICAL SOC
Citation statistics
Cited Times:2[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/172044
Collection中国科学院大连化学物理研究所
Corresponding AuthorLi, Xingwei
Affiliation1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
2.Shaanxi Normal Univ SNNU, Sch Chem & Chem Engn, Xian 710062, Shaanxi, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
Recommended Citation
GB/T 7714
Xu, Youwei,Zheng, Guangfan,Kong, Lingheng,et al. Manganese(I)-Catalyzed Synthesis of Fused Eight- and Four-Membered Carbocycles via C-H Activation and Pericyclic Reactions[J]. ORGANIC LETTERS,2019,21(9):3402-3406.
APA Xu, Youwei,Zheng, Guangfan,Kong, Lingheng,&Li, Xingwei.(2019).Manganese(I)-Catalyzed Synthesis of Fused Eight- and Four-Membered Carbocycles via C-H Activation and Pericyclic Reactions.ORGANIC LETTERS,21(9),3402-3406.
MLA Xu, Youwei,et al."Manganese(I)-Catalyzed Synthesis of Fused Eight- and Four-Membered Carbocycles via C-H Activation and Pericyclic Reactions".ORGANIC LETTERS 21.9(2019):3402-3406.
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