DICP OpenIR
Recent Progress in Catalytic Oxidative Transformations of Alcohols by Supported Gold Nanoparticles
Hui, Yonghai1; Zhang, Shiqi1; Wang, Wentao2
Corresponding AuthorWang, Wentao(wentaowang@dicp.ac.cn)
Keywordalcohols aldehydes gold nanoparticles heterogeneous catalysis ketones oxidation
Source PublicationADVANCED SYNTHESIS & CATALYSIS
2019-05-14
ISSN1615-4150
DOI10.1002/adsc.201801595
Volume361Issue:10Pages:2215-2235
Funding ProjectNational Natural Science Foundation of China[21672210] ; Doctoral Fund of Lingnan Normal University[ZL1817]
Funding OrganizationNational Natural Science Foundation of China ; National Natural Science Foundation of China ; Doctoral Fund of Lingnan Normal University ; Doctoral Fund of Lingnan Normal University ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Doctoral Fund of Lingnan Normal University ; Doctoral Fund of Lingnan Normal University ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Doctoral Fund of Lingnan Normal University ; Doctoral Fund of Lingnan Normal University ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Doctoral Fund of Lingnan Normal University ; Doctoral Fund of Lingnan Normal University
WOS SubjectChemistry, Applied ; Chemistry, Organic
WOS Research AreaChemistry
WOS KeywordSOLVENT-FREE OXIDATION ; SELECTIVE AEROBIC OXIDATION ; METAL-ORGANIC FRAMEWORKS ; HIGHLY EFFICIENT ; BENZYL ALCOHOL ; MOLECULAR-OXYGEN ; AU NANOPARTICLES ; STEP SYNTHESIS ; ETHANOL ; HYDROTALCITE
AbstractCatalytic oxidative transformations of alcohols constitute one of the greatly important protocols for the synthesis of various aldehydes, ketones, acids, imines, amides, etc. that are required to make drug intermediates, food additives, plastics, detergents and cosmetics. The potential of gold nanoparticles (Au NPs) in catalytic oxidation reactions is generally competent owing to their tendency to activate oxygen. Supports play a conspicuous and increasingly important role not only in the preparation and stabilization of Au NPs, but also can address the issues of sustainability by facilitating separation and reusability of the catalyst. This review aims to systematically discuss the impressive developments in catalytic oxidative transformations of alcohols promoted by supported Au NPs in the last five years. These Au NPs exhibit unique electronic properties and crystal structures, which gives us an excellent opportunity to correlate atomic structure with intrinsic catalytic properties over Au NPs. The effect of a support on the significant properties of Au NPs in terms of catalytic activity, selectivity, recyclability, and stability is discussed at length. The tentative reaction mechanisms and the structure-performance relationships are also discussed at appropriate places, which will provide some clues for the design of efficient Au NPs-based catalysts.
Language英语
Funding OrganizationNational Natural Science Foundation of China ; National Natural Science Foundation of China ; Doctoral Fund of Lingnan Normal University ; Doctoral Fund of Lingnan Normal University ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Doctoral Fund of Lingnan Normal University ; Doctoral Fund of Lingnan Normal University ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Doctoral Fund of Lingnan Normal University ; Doctoral Fund of Lingnan Normal University ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Doctoral Fund of Lingnan Normal University ; Doctoral Fund of Lingnan Normal University
WOS IDWOS:000471326000002
PublisherWILEY-V C H VERLAG GMBH
Citation statistics
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/172068
Collection中国科学院大连化学物理研究所
Corresponding AuthorWang, Wentao
Affiliation1.Lingnan Normal Univ, Coll Chem & Chem Engn, Zhanjiang 524048, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
Recommended Citation
GB/T 7714
Hui, Yonghai,Zhang, Shiqi,Wang, Wentao. Recent Progress in Catalytic Oxidative Transformations of Alcohols by Supported Gold Nanoparticles[J]. ADVANCED SYNTHESIS & CATALYSIS,2019,361(10):2215-2235.
APA Hui, Yonghai,Zhang, Shiqi,&Wang, Wentao.(2019).Recent Progress in Catalytic Oxidative Transformations of Alcohols by Supported Gold Nanoparticles.ADVANCED SYNTHESIS & CATALYSIS,361(10),2215-2235.
MLA Hui, Yonghai,et al."Recent Progress in Catalytic Oxidative Transformations of Alcohols by Supported Gold Nanoparticles".ADVANCED SYNTHESIS & CATALYSIS 361.10(2019):2215-2235.
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