DICP OpenIR
Scalable Ambient Fabrication of High-Performance CsPbI2Br Solar Cells
Fan, Yuanyuan1,2,3; Fang, Junjie1,2,3; Chang, Xiaoming1,2,3; Tang, Ming-Chun5,6; Barrit, Dounya5,6; Xu, Zhuo1,2,3; Jiang, Zhiwu7; Wen, Jialun1,2,3; Zhao, Huan1,2,3; Niu, Tianqi1,2,3; Smilgies, Detlef-M8; Jin, Shengye4; Liu, Zhike1,2,3; Li, Er Qiang7; Amassian, Aram5,6,9; Liu, Shengzhong (Frank)1,2,3,4; Zhao, Kui1,2,3
Corresponding AuthorAmassian, Aram(aamassi@ncsu.edu) ; Liu, Shengzhong (Frank)(szliu@dicp.ac.cn) ; Zhao, Kui(zhaok@snnu.edu.cn)
Source PublicationJOULE
2019-10-16
ISSN2542-4351
DOI10.1016/j.joule.2019.07.015
Volume3Issue:10Pages:2485-2502
Funding ProjectNational Key Research and Development Program of China[2017YFA0204800] ; National Key Research and Development Program of China[2016YFA0202403] ; National Natural Science Foundation of China[61604092] ; National Natural Science Foundation of China[11772327] ; National Natural Science Foundation of China[11621202] ; DNL Cooperation Fund CAS[DNL180311] ; National University Research Fund[GK201802005] ; 111 Project[B14041] ; National 1000 Talents Plan program[1110010341] ; King Abdullah University of Science and Technology (KAUST) ; NSF[DMR-1332208]
Funding OrganizationNational Key Research and Development Program of China ; National Key Research and Development Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; DNL Cooperation Fund CAS ; DNL Cooperation Fund CAS ; National University Research Fund ; National University Research Fund ; 111 Project ; 111 Project ; National 1000 Talents Plan program ; National 1000 Talents Plan program ; King Abdullah University of Science and Technology (KAUST) ; King Abdullah University of Science and Technology (KAUST) ; NSF ; NSF ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; DNL Cooperation Fund CAS ; DNL Cooperation Fund CAS ; National University Research Fund ; National University Research Fund ; 111 Project ; 111 Project ; National 1000 Talents Plan program ; National 1000 Talents Plan program ; King Abdullah University of Science and Technology (KAUST) ; King Abdullah University of Science and Technology (KAUST) ; NSF ; NSF ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; DNL Cooperation Fund CAS ; DNL Cooperation Fund CAS ; National University Research Fund ; National University Research Fund ; 111 Project ; 111 Project ; National 1000 Talents Plan program ; National 1000 Talents Plan program ; King Abdullah University of Science and Technology (KAUST) ; King Abdullah University of Science and Technology (KAUST) ; NSF ; NSF ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; DNL Cooperation Fund CAS ; DNL Cooperation Fund CAS ; National University Research Fund ; National University Research Fund ; 111 Project ; 111 Project ; National 1000 Talents Plan program ; National 1000 Talents Plan program ; King Abdullah University of Science and Technology (KAUST) ; King Abdullah University of Science and Technology (KAUST) ; NSF ; NSF
WOS SubjectChemistry, Physical ; Energy & Fuels ; Materials Science, Multidisciplinary
WOS Research AreaChemistry ; Energy & Fuels ; Materials Science
WOS KeywordPATTERN-FORMATION ; PEROVSKITE FILMS ; HIGH-EFFICIENCY ; SURFACE ; DEGRADATION ; DEPOSITION
AbstractAll-inorganic halide perovskites hold promise for emerging thin-film photovoltaics due to their excellent thermal stability. Unfortunately, it has been challenging to achieve high-quality films over large areas using scalable methods under realistic ambient conditions. Herein, we investigated the coupling between the fluid dynamics and the structural evolution during controlled film formation for ambient scalable fabrication of CsPbl(2)Br perovskite films using blade coating. We simultaneously overcame the negative influences of moisture attack and the Benard-Marangoni instability in the drying ink and achieved an ideal sequential crystallization with changing halide composition during the film formation. As a result, we produced highly crystalline, uniform, and pinhole-free CsPbl(2)Br films with superior photophysical and transport properties. High-performance solar cells are fabricated to achieve power conversion efficiencies (PCEs) of 14.7% for small-aperture-area (0.03 cm(2)) devices and 12.5% for the large-aperture-area (1.0 cm(2)) ones, the highest PCE reported to date for large-area all-inorganic perovskite solar cells.
Language英语
Funding OrganizationNational Key Research and Development Program of China ; National Key Research and Development Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; DNL Cooperation Fund CAS ; DNL Cooperation Fund CAS ; National University Research Fund ; National University Research Fund ; 111 Project ; 111 Project ; National 1000 Talents Plan program ; National 1000 Talents Plan program ; King Abdullah University of Science and Technology (KAUST) ; King Abdullah University of Science and Technology (KAUST) ; NSF ; NSF ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; DNL Cooperation Fund CAS ; DNL Cooperation Fund CAS ; National University Research Fund ; National University Research Fund ; 111 Project ; 111 Project ; National 1000 Talents Plan program ; National 1000 Talents Plan program ; King Abdullah University of Science and Technology (KAUST) ; King Abdullah University of Science and Technology (KAUST) ; NSF ; NSF ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; DNL Cooperation Fund CAS ; DNL Cooperation Fund CAS ; National University Research Fund ; National University Research Fund ; 111 Project ; 111 Project ; National 1000 Talents Plan program ; National 1000 Talents Plan program ; King Abdullah University of Science and Technology (KAUST) ; King Abdullah University of Science and Technology (KAUST) ; NSF ; NSF ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; DNL Cooperation Fund CAS ; DNL Cooperation Fund CAS ; National University Research Fund ; National University Research Fund ; 111 Project ; 111 Project ; National 1000 Talents Plan program ; National 1000 Talents Plan program ; King Abdullah University of Science and Technology (KAUST) ; King Abdullah University of Science and Technology (KAUST) ; NSF ; NSF
WOS IDWOS:000490703300020
PublisherCELL PRESS
Citation statistics
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/172295
Collection中国科学院大连化学物理研究所
Corresponding AuthorAmassian, Aram; Liu, Shengzhong (Frank); Zhao, Kui
Affiliation1.Shaanxi Normal Univ, Key Lab Appl Surface & Colloid Chem, Minist Educ, Xian 710119, Shaanxi, Peoples R China
2.Shaanxi Normal Univ, Shaanxi Key Lab Adv Energy Devices, Xian 710119, Shaanxi, Peoples R China
3.Shaanxi Normal Univ, Shaanxi Engn Lab Adv Energy Technol, Sch Mat Sci & Engn, Xian 710119, Shaanxi, Peoples R China
4.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, iChEM, Dalian 116023, Peoples R China
5.KAUST, KSC, Thuwal 239556900, Saudi Arabia
6.KAUST, Phys Sci & Engn Div PSE, Thuwal 239556900, Saudi Arabia
7.Univ Sci & Technol China, Dept Modern Mech, Hefei 230027, Anhui, Peoples R China
8.Cornell Univ, Cornell High Energy Synchrotron Source, Ithaca, NY 14850 USA
9.North Carolina State Univ, Dept Mat Sci & Engn, Raleigh, NC 27695 USA
Recommended Citation
GB/T 7714
Fan, Yuanyuan,Fang, Junjie,Chang, Xiaoming,et al. Scalable Ambient Fabrication of High-Performance CsPbI2Br Solar Cells[J]. JOULE,2019,3(10):2485-2502.
APA Fan, Yuanyuan.,Fang, Junjie.,Chang, Xiaoming.,Tang, Ming-Chun.,Barrit, Dounya.,...&Zhao, Kui.(2019).Scalable Ambient Fabrication of High-Performance CsPbI2Br Solar Cells.JOULE,3(10),2485-2502.
MLA Fan, Yuanyuan,et al."Scalable Ambient Fabrication of High-Performance CsPbI2Br Solar Cells".JOULE 3.10(2019):2485-2502.
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