DICP OpenIR
Aliphatic amines modified CoO nanoparticles for catalytic oxidation of aromatic hydrocarbon with molecular oxygen
Liu, Meng1,2; Shi, Song1; Zhao, Li1,2; Chen, Chen1,3; Gao, Jin1; Xu, Jie1
Corresponding AuthorShi, Song(shisong@dicp.ac.cn) ; Xu, Jie(xujie@dicp.ac.cn)
KeywordHydrocarbon oxidation Hydrophobic modification Amines coating Cobalt oxide Surface modification
Source PublicationCHINESE JOURNAL OF CATALYSIS
2019-10-01
ISSN0253-9837
DOI10.1016/S1872-2067(19)63413-3
Volume40Issue:10Pages:1488-1493
Funding ProjectNational Natural Science Foundation of China[21790331] ; National Natural Science Foundation of China[21603218] ; Strategic Priority Research Program of Chinese Academy of Sciences[XDA21030400] ; Strategic Priority Research Program of Chinese Academy of Sciences[XDB17020300]
Funding OrganizationNational Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Strategic Priority Research Program of Chinese Academy of Sciences ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Strategic Priority Research Program of Chinese Academy of Sciences ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Strategic Priority Research Program of Chinese Academy of Sciences ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Strategic Priority Research Program of Chinese Academy of Sciences
WOS SubjectChemistry, Applied ; Chemistry, Physical ; Engineering, Chemical
WOS Research AreaChemistry ; Engineering
WOS KeywordSELECTIVE OXIDATION ; REDUCING AGENT ; ETHYLBENZENE ; NANOCRYSTALS ; CYCLOHEXANE ; PERFORMANCE ; OLEYLAMINE ; COBALT ; OXIDES ; CO3O4
AbstractThe surface modification of metal oxides using organic modifiers is a potential strategy for enhancing their catalytic performances. In this study, a hydrophobic surface amine-modified CoO catalyst with a water contact angle of 143 was fabricated. The catalyst was characterized by XRD, TGA, FT-IR, HR-TEM, and XPS. The results showed that the fabricated catalyst performed better than the hydrophilic commercial CoO nanoparticle in the process of aromatic hydrocarbon oxidation. After the amines modification, commercial CoO also became hydrophobic and improved conversion of ethylbenzene was achieved. The surface modification of CoO with amines induced the hydrophobicity property, which could serve as a reference for the design of other hydrophobic catalysts. (C) 2019, Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier B.V. All rights reserved.
Language英语
Funding OrganizationNational Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Strategic Priority Research Program of Chinese Academy of Sciences ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Strategic Priority Research Program of Chinese Academy of Sciences ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Strategic Priority Research Program of Chinese Academy of Sciences ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Strategic Priority Research Program of Chinese Academy of Sciences
WOS IDWOS:000490625200005
PublisherSCIENCE PRESS
Citation statistics
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/172494
Collection中国科学院大连化学物理研究所
Corresponding AuthorShi, Song; Xu, Jie
Affiliation1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian Natl Lab Clean Energy, Dalian 116023, Liaoning, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.Ningbo Univ, Sch Mat Sci & Chem Engn, Ningbo 315211, Zhejiang, Peoples R China
Recommended Citation
GB/T 7714
Liu, Meng,Shi, Song,Zhao, Li,et al. Aliphatic amines modified CoO nanoparticles for catalytic oxidation of aromatic hydrocarbon with molecular oxygen[J]. CHINESE JOURNAL OF CATALYSIS,2019,40(10):1488-1493.
APA Liu, Meng,Shi, Song,Zhao, Li,Chen, Chen,Gao, Jin,&Xu, Jie.(2019).Aliphatic amines modified CoO nanoparticles for catalytic oxidation of aromatic hydrocarbon with molecular oxygen.CHINESE JOURNAL OF CATALYSIS,40(10),1488-1493.
MLA Liu, Meng,et al."Aliphatic amines modified CoO nanoparticles for catalytic oxidation of aromatic hydrocarbon with molecular oxygen".CHINESE JOURNAL OF CATALYSIS 40.10(2019):1488-1493.
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