DICP OpenIR
Ru/H-beta as an efficient catalyst for the conversion of furfural into 3-acetyl-1-propanol (3-AP) toward one-pot transformation of xylan to 3-AP
Liu, Qiaoyun1; Liu, Fei1; Zhang, Yaru1,3; Su, Yang1; Wang, Aiqin1,2; Zhang, Tao1,2
Corresponding AuthorLiu, Fei() ; Zhang, Tao(taozhang@dicp.ac.cn)
KeywordBiomass Furfural 3-acetyl-1-propanol Carbohydrates Ru-based bifunctional catalysts
Source PublicationMOLECULAR CATALYSIS
2019-10-01
ISSN2468-8231
DOI10.1016/j.mcat.2019.110506
Volume476Pages:6
Funding ProjectNational Key Projects for Fundamental Research and Development of China[2018YF1501602] ; National Key Projects for Fundamental Research and Development of China[2016YFA0202801] ; National Natural Science Foundation of China[21606227] ; National Natural Science Foundation of China[21690080] ; National Natural Science Foundation of China[21690084] ; National Natural Science Foundation of China[21721004] ; National Natural Science Foundation of China[21673228] ; Strategic Priority Research Program of the Chinese Academy of Sciences[XDB17020100] ; Dalian National Laboratory for Clean Energy[DNL180303]
Funding OrganizationNational Key Projects for Fundamental Research and Development of China ; National Key Projects for Fundamental Research and Development of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Dalian National Laboratory for Clean Energy ; Dalian National Laboratory for Clean Energy ; National Key Projects for Fundamental Research and Development of China ; National Key Projects for Fundamental Research and Development of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Dalian National Laboratory for Clean Energy ; Dalian National Laboratory for Clean Energy ; National Key Projects for Fundamental Research and Development of China ; National Key Projects for Fundamental Research and Development of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Dalian National Laboratory for Clean Energy ; Dalian National Laboratory for Clean Energy ; National Key Projects for Fundamental Research and Development of China ; National Key Projects for Fundamental Research and Development of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Dalian National Laboratory for Clean Energy ; Dalian National Laboratory for Clean Energy
WOS SubjectChemistry, Physical
WOS Research AreaChemistry
WOS KeywordSELECTIVE OXIDATION ; ALCOHOLS ; SOLVENT ; 1,5-PENTANEDIOL ; HYDROGENATION ; CHEMICALS ; PLATFORM ; ALKANES ; WATER ; ACID
AbstractA highly active and robust catalyst composed of Ru nanoparticles highly dispersed on zeolite H-beta was developed for transforming furfural into 3-acetyl-1-propanol (3-AP) in good yield (81%)under mild conditions (80 degrees C, 1 MPa H-2). Both the support nature and the preparation methods had significant impacts on the dispersion of Ru, eventually on the yield of 3-AP. Ion-exchange method proved best for obtaining the highly active and selective catalyst for this reaction. Moreover, the catalyst can be regenerated easily by calcination and reduction. This catalyst was further explored for the one-pot conversion of xylose and xylan to 3-AP with a yield of 46% and 31%, respectively, thus opening a new feasible pathway from biomass to valuable fine chemicals.
Language英语
Funding OrganizationNational Key Projects for Fundamental Research and Development of China ; National Key Projects for Fundamental Research and Development of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Dalian National Laboratory for Clean Energy ; Dalian National Laboratory for Clean Energy ; National Key Projects for Fundamental Research and Development of China ; National Key Projects for Fundamental Research and Development of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Dalian National Laboratory for Clean Energy ; Dalian National Laboratory for Clean Energy ; National Key Projects for Fundamental Research and Development of China ; National Key Projects for Fundamental Research and Development of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Dalian National Laboratory for Clean Energy ; Dalian National Laboratory for Clean Energy ; National Key Projects for Fundamental Research and Development of China ; National Key Projects for Fundamental Research and Development of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Dalian National Laboratory for Clean Energy ; Dalian National Laboratory for Clean Energy
WOS IDWOS:000488661800019
PublisherELSEVIER
Citation statistics
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/172602
Collection中国科学院大连化学物理研究所
Corresponding AuthorLiu, Fei; Zhang, Tao
Affiliation1.Chinese Acad Sci, Key Lab Sci & Technol Appl Catalysis, Dalian 116023, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
Recommended Citation
GB/T 7714
Liu, Qiaoyun,Liu, Fei,Zhang, Yaru,et al. Ru/H-beta as an efficient catalyst for the conversion of furfural into 3-acetyl-1-propanol (3-AP) toward one-pot transformation of xylan to 3-AP[J]. MOLECULAR CATALYSIS,2019,476:6.
APA Liu, Qiaoyun,Liu, Fei,Zhang, Yaru,Su, Yang,Wang, Aiqin,&Zhang, Tao.(2019).Ru/H-beta as an efficient catalyst for the conversion of furfural into 3-acetyl-1-propanol (3-AP) toward one-pot transformation of xylan to 3-AP.MOLECULAR CATALYSIS,476,6.
MLA Liu, Qiaoyun,et al."Ru/H-beta as an efficient catalyst for the conversion of furfural into 3-acetyl-1-propanol (3-AP) toward one-pot transformation of xylan to 3-AP".MOLECULAR CATALYSIS 476(2019):6.
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