DICP OpenIR
Single Atom Alloy Preparation and Applications in Heterogeneous Catalysis
Han, Jianyu1,2; Lu, Jianmin1; Wang, Min3; Wang, Yehong1; Wang, Feng1
Corresponding AuthorWang, Feng(wangfeng@dicp.ac.cn)
Source PublicationCHINESE JOURNAL OF CHEMISTRY
2019-08-01
ISSN1001-604X
DOI10.1002/cjoc.201900185
Pages12
Funding ProjectNational Natural Science Foundation of China[21721004] ; National Natural Science Foundation of China[21711530020] ; National Natural Science Foundation of China[21690082] ; National Natural Science Foundation of China[21690084] ; National Natural Science Foundation of China[21690080] ; Strategic Priority Research Program of Chinese Academy of Sciences[XDB17020300] ; Strategic Priority Research Program of Chinese Academy of Sciences[XDB17000000]
Funding OrganizationNational Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Strategic Priority Research Program of Chinese Academy of Sciences ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Strategic Priority Research Program of Chinese Academy of Sciences ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Strategic Priority Research Program of Chinese Academy of Sciences ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Strategic Priority Research Program of Chinese Academy of Sciences
WOS SubjectChemistry, Multidisciplinary
WOS Research AreaChemistry
WOS KeywordSELECTIVE HYDROGENATION ; GOLD-NANOCLUSTERS ; ELECTRONIC-STRUCTURE ; CRYSTAL-STRUCTURE ; OPTICAL-PROPERTIES ; MASS-SPECTROMETRY ; CO OXIDATION ; PD ; SURFACE ; AU-25
AbstractThere have been remarkable progresses in manipulating heterogeneous catalysts' nanostructures in the past decade. The concept of single atom alloy (SAA) was firstly proposed in 2012 when researchers successfully stabilized single Pd atoms on the Cu(111) surface. However, earlier work in 2009, which focused on replacing one Au atom with a Pd atom in thiolate protected Au-25 nanoclusters, could also be considered as the pioneer work of single atom alloy. Both kinds of single atom alloys exhibited the potential of maximum utilization of scarce elements and attractive catalytic performances. The well-defined structures of SAA catalysts make accurate modeling possible, which further realizes the rational design of single atom alloy catalysts. In this review, we summarize the research trajectory of single atom alloys as well as recent achievements in this field. We also introduce several commonly adopted characterization methods for SAA catalysts such as scanning tunneling microscopy (STM), temperature programmed reaction (TPR), extended X-ray absorption fine structure (EXAFS) spectra, matrix assisted laser desorption/ionization mass spectrum (MALDI-MS) and differential pulse voltammetry (DPV). Through discussing recent progresses in SAA catalysts, we propose that future researches in this filed should be focused on exploring new kinds of metal nanocrystals and controlling the nanostructure of SAA even more precisely.
Language英语
Funding OrganizationNational Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Strategic Priority Research Program of Chinese Academy of Sciences ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Strategic Priority Research Program of Chinese Academy of Sciences ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Strategic Priority Research Program of Chinese Academy of Sciences ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Strategic Priority Research Program of Chinese Academy of Sciences
WOS IDWOS:000479834700001
PublisherWILEY-V C H VERLAG GMBH
Citation statistics
Cited Times:2[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/173422
Collection中国科学院大连化学物理研究所
Corresponding AuthorWang, Feng
Affiliation1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian Natl Lab Clean Energy, State Key Lab Catalysis, Dalian 116023, Liaoning, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.Dalian Univ Technol, Zhang Dayu Sch Chem, Dalian 116024, Liaoning, Peoples R China
Recommended Citation
GB/T 7714
Han, Jianyu,Lu, Jianmin,Wang, Min,et al. Single Atom Alloy Preparation and Applications in Heterogeneous Catalysis[J]. CHINESE JOURNAL OF CHEMISTRY,2019:12.
APA Han, Jianyu,Lu, Jianmin,Wang, Min,Wang, Yehong,&Wang, Feng.(2019).Single Atom Alloy Preparation and Applications in Heterogeneous Catalysis.CHINESE JOURNAL OF CHEMISTRY,12.
MLA Han, Jianyu,et al."Single Atom Alloy Preparation and Applications in Heterogeneous Catalysis".CHINESE JOURNAL OF CHEMISTRY (2019):12.
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