DICP OpenIR
Decorated Traditional Zeolites with Subunits of Metal-Organic Frameworks for CH4/N-2 Separation
Wu, Yaqi1,2; Yuan, Danhua1; He, Dawei1,2; Xing, Jiacheng1,2; Zeng, Shu1,2; Xu, Shutao1; Xu, Yunpeng1; Liu, Zhongmin1
Corresponding AuthorXu, Yunpeng(xuyp@dicp.ac.cn) ; Liu, Zhongmin(liuzm@dicp.ac.cn)
Keywordgas adsorption metal-organic frameworks surface decoration zeolites
Source PublicationANGEWANDTE CHEMIE-INTERNATIONAL EDITION
2019-07-22
ISSN1433-7851
DOI10.1002/anie.201905014
Volume58Issue:30Pages:10241-10244
Funding ProjectNational Key Research and Development Program of China[2016YFB0301603]
Funding OrganizationNational Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China
WOS SubjectChemistry, Multidisciplinary
WOS Research AreaChemistry
WOS KeywordIMIDAZOLATE FRAMEWORKS ; NMR ; ADSORPTION ; ZIF-8 ; CO2 ; TEMPERATURE ; MEMBRANES ; MOBILITY ; DESIGN ; XENON
AbstractMetal-organic frameworks (MOF) materials are promising materials for gas separation, but their application still faces various challenges. A strategy is now reported for introducing subunits of MOFs into traditional zeolite frameworks to obtain applicable adsorbents with advantages of both zeolites and MOFs. The subunits of ZIFs were introduced into zeolite Y and zeolite ZSM-5 for CH4/N-2 separation. Both the molecular simulation and experimental results validated that the IAST CH4/N-2 selectivity of the resulting samples greatly improved (above 8, at 100 kPa and 25 degrees C) with the incorporation of ZIF subunits into zeolites structure, and the selectivities were obviously higher than that of zeolites and even better than that of ZIFs. This strategy not only gave rise to an efficient adsorbent for CH4/N-2 separation but also provided ideas for design of other adsorption and separation materials.
Language英语
Funding OrganizationNational Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China
WOS IDWOS:000476452700032
PublisherWILEY-V C H VERLAG GMBH
Citation statistics
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/173969
Collection中国科学院大连化学物理研究所
Corresponding AuthorXu, Yunpeng; Liu, Zhongmin
Affiliation1.Chinese Acad Sci, Dalian Inst Chem Phys, Natl Engn Lab Methanol Olefins, Dalian Natl Lab Clean Energy, Dalian 116023, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
Recommended Citation
GB/T 7714
Wu, Yaqi,Yuan, Danhua,He, Dawei,et al. Decorated Traditional Zeolites with Subunits of Metal-Organic Frameworks for CH4/N-2 Separation[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2019,58(30):10241-10244.
APA Wu, Yaqi.,Yuan, Danhua.,He, Dawei.,Xing, Jiacheng.,Zeng, Shu.,...&Liu, Zhongmin.(2019).Decorated Traditional Zeolites with Subunits of Metal-Organic Frameworks for CH4/N-2 Separation.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,58(30),10241-10244.
MLA Wu, Yaqi,et al."Decorated Traditional Zeolites with Subunits of Metal-Organic Frameworks for CH4/N-2 Separation".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION 58.30(2019):10241-10244.
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