DICP OpenIR
The Evolution in Catalytic Activity Driven by Periodic Transformation in the Inner Sites of Gold Clusters
Sun, Yongnan1; Wang, Endong2; Ren, Yujing3; Xiao, Kang4; Liu, Xu1; Yang, Dan1; Gao, Yi2; Ding, Weiping1; Zhu, Yan1
Corresponding AuthorGao, Yi(gaoyi@sinap.ac.cn) ; Zhu, Yan(zhuyan@nju.edu.cn)
Keywordactivity evolution gold clusters inner sites periodic structure
Source PublicationADVANCED FUNCTIONAL MATERIALS
2019-07-11
ISSN1616-301X
DOI10.1002/adfm.201904242
Pages8
Funding ProjectNational Natural Science Foundation of China[21773109] ; National Natural Science Foundation of China[21773287] ; National Natural Science Foundation of China[91845104] ; Fundamental Research Funds for the Central Universities
Funding OrganizationNational Natural Science Foundation of China ; National Natural Science Foundation of China ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities
WOS SubjectChemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
WOS Research AreaChemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
WOS KeywordBONDING PROPERTIES ; CO OXIDATION ; NANOCLUSTERS ; TEMPERATURE ; ALKYNES ; COMPLEXES ; LIGANDS ; SN
AbstractIt is extremely difficult to distinguish the contributions of different sites on the surface and in the inner sites of a catalyst to the overall catalytic performance, as the observed catalytic results reflect an ensemble average from almost all the active sites. How do the inner sites of a catalyst that seem to be not directly involved in a catalytic process exactly contribute to the catalytic performance? Toward this goal, herein the studies not only provide fundamental insights into how the alteration of Au8n+4(SR)(4n+8) clusters by only the inner structure can dramatically change the intrinsic catalytic properties, where Au8n+4(SR)(4n+8) (n = 3, 4, 5) clusters have the same surface motifs but share a periodic kernel structure, but also further demonstrate that the evolution in catalytic activity can potentially be determined by periodic transformation in the inner kernels.
Language英语
Funding OrganizationNational Natural Science Foundation of China ; National Natural Science Foundation of China ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Fundamental Research Funds for the Central Universities ; Fundamental Research Funds for the Central Universities
WOS IDWOS:000474959000001
PublisherWILEY-V C H VERLAG GMBH
Citation statistics
Cited Times:2[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/175606
Collection中国科学院大连化学物理研究所
Corresponding AuthorGao, Yi; Zhu, Yan
Affiliation1.Nanjing Univ, Sch Chem & Chem Engn, Nanjing 210093, Jiangsu, Peoples R China
2.Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China
3.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
4.Nanjing Univ Posts & Telecommun, Sch Mat Sci & Engn, Nanjing 210023, Jiangsu, Peoples R China
Recommended Citation
GB/T 7714
Sun, Yongnan,Wang, Endong,Ren, Yujing,et al. The Evolution in Catalytic Activity Driven by Periodic Transformation in the Inner Sites of Gold Clusters[J]. ADVANCED FUNCTIONAL MATERIALS,2019:8.
APA Sun, Yongnan.,Wang, Endong.,Ren, Yujing.,Xiao, Kang.,Liu, Xu.,...&Zhu, Yan.(2019).The Evolution in Catalytic Activity Driven by Periodic Transformation in the Inner Sites of Gold Clusters.ADVANCED FUNCTIONAL MATERIALS,8.
MLA Sun, Yongnan,et al."The Evolution in Catalytic Activity Driven by Periodic Transformation in the Inner Sites of Gold Clusters".ADVANCED FUNCTIONAL MATERIALS (2019):8.
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