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Methanol synthesis from CO2 using a silicone rubber/ceramic composite membrane reactor
Chen, GW; Yuan, Q
关键词Co2 Hydrogenation Damkohler Number Fixed Bed Reactor Membrane Separation Factor Non-uniform Permeation
刊名SEPARATION AND PURIFICATION TECHNOLOGY
2004
DOI10.1016/S1383-5866(03)00195-3
34期:1-3页:227-237
收录类别ISTP ; SCI
文章类型Article
项目归属903
产权排名1;1
WOS标题词Science & Technology ; Technology
类目[WOS]Engineering, Chemical
研究领域[WOS]Engineering
关键词[WOS]DEHYDROGENATION ; SEPARATION ; OXIDATION ; ETHANE
英文摘要A one-dimensional isothermal pseudo-homogeneous parallel flow model was developed for the methanol synthesis from CO2 in a silicone rubber/ceramic composite membrane reactor. The fourth-order Runge-Kutta method was adopted to simulate the process behaviors in the membrane reactor. How those parameters affect the reaction behaviors in the membrane reactor, such as Damkohler number Da, pressure ratio p(r), reaction temperature T, membrane separation factor alpha, membrane permeation parameter phi , as well as the non-uniform parameter of membrane permeation L-1, were discussed in detail. Parts of the theoretical results were tested and verified; the experimental results showed that the conversion of the main reaction in the membrane reactor increased by 22% against traditional fixed bed reactor, and the optimal non-uniform parameter of membrane permeation rate, L-1.opt ,does exist. (C) 2003 Elsevier B.V All rights reserved.
语种英语
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WOS记录号WOS:000188537500027
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被引频次:19[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/81019
专题中国科学院大连化学物理研究所
作者单位Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
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GB/T 7714
Chen, GW,Yuan, Q. Methanol synthesis from CO2 using a silicone rubber/ceramic composite membrane reactor[J]. SEPARATION AND PURIFICATION TECHNOLOGY,2004,34(1-3):227-237.
APA Chen, GW,&Yuan, Q.(2004).Methanol synthesis from CO2 using a silicone rubber/ceramic composite membrane reactor.SEPARATION AND PURIFICATION TECHNOLOGY,34(1-3),227-237.
MLA Chen, GW,et al."Methanol synthesis from CO2 using a silicone rubber/ceramic composite membrane reactor".SEPARATION AND PURIFICATION TECHNOLOGY 34.1-3(2004):227-237.
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