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题名: Autler-townes splitting in the multiphoton resonance ionization spectrum of molecules produced by ultrashort laser pulses
作者: Sun, ZG;  Lou, NQ
刊名: PHYSICAL REVIEW LETTERS
发表日期: 2003-07-11
DOI: 10.1103/PhysRevLett.91.023002
卷: 91, 期:2, 页:023002-1-023002-4
收录类别: SCI
文章类型: Article
部门归属: 1102
项目归属: 1102
产权排名: 1;1
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Physics, Multidisciplinary
研究领域[WOS]: Physics
英文摘要: We report for the first time the proper conditions to observe Autler-Townes splitting (ac-Stark splitting) from vibrationally coherent states belonging to the different electronic terms of a diatomic molecule. Wave packet dynamics simulations demonstrate that such a process is feasible by multiphoton resonance ionization of the molecule Na-2 with a single ultrashort intense laser pulse. With the ultrahigh time resolution of a femtosecond laser pulse, one can directly measure the absolute value of the transition dipole moment between any kinds of molecular states by this kind of Autler-Townes splitting, which is a function of the internuclear distance R.
关键词[WOS]: LIGHT-INDUCED POTENTIALS ;  TRANSITION MOMENTS ;  STARK SHIFT ;  FEMTOSECOND ;  STATES ;  DYNAMICS ;  FIELDS ;  NA-2 ;  CURVES ;  DIPOLE
语种: 英语
原文出处: 查看原文
WOS记录号: WOS:000184086000014
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/82463
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China

Recommended Citation:
Sun, ZG,Lou, NQ. Autler-townes splitting in the multiphoton resonance ionization spectrum of molecules produced by ultrashort laser pulses[J]. PHYSICAL REVIEW LETTERS,2003,91(2):023002-1-023002-4.
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