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题名: Direct conversion of methane under nonoxidative conditions
作者: Xu, YD;  Bao, XH;  Lin, LW
关键词: direct conversion of methane ;  nonoxidative condition ;  dehydroaromatization ;  Mo/HZSM-5 ;  bifunctionality ;  carbonaceous deposits
刊名: JOURNAL OF CATALYSIS
发表日期: 2003-05-15
DOI: 10.1016/S0021-9517(02)00124-0
卷: 216, 期:1-2, 页:386-395
收录类别: SCI
文章类型: Article
部门归属: 501
项目归属: 501
产权排名: 1;1
WOS标题词: Science & Technology ;  Physical Sciences ;  Technology
类目[WOS]: Chemistry, Physical ;  Engineering, Chemical
研究领域[WOS]: Chemistry ;  Engineering
英文摘要: Direct conversion of methane into hydrogen and valuable chemicals under nonoxidative conditions is a process severely limited thermodynamically. However, the movement from the present era of fossil fuels into the coming hydrogen energy age makes it an interesting and important approach compared with the direct conversion of methane under the aid of oxidants. This paper gives a brief overview of the direct conversion of CH4 under nonoxidative conditions. At the same time, our understanding of methane dehydroaromatization over Mo/HZSM-5 catalysts for the simultaneous formation of hydrogen and light aromatics is discussed in general, while the bifunctionality of Mo/HZSM-5 catalysts and the role of carbonaceous deposits formed during the reaction are reviewed in more detail. A perspective of the topic from both academic points of view and potential industrial applications is also presented. (C) 2003 Elsevier Science (USA). All rights reserved.
关键词[WOS]: OXYGEN-FREE CONVERSION ;  ISOTHERMAL 2-STEP REACTION ;  PT-CO/NAY CATALYSTS ;  MO-BASED CATALYSTS ;  HIGHER HYDROCARBONS ;  REACTION SEQUENCE ;  LOW-TEMPERATURE ;  HIGHER ALKANES ;  ELECTROPHILIC REACTIONS ;  BIFUNCTIONAL CATALYSIS
语种: 英语
原文出处: 查看原文
WOS记录号: WOS:000183226900036
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/82861
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China

Recommended Citation:
Xu, YD,Bao, XH,Lin, LW. Direct conversion of methane under nonoxidative conditions[J]. JOURNAL OF CATALYSIS,2003,216(1-2):386-395.
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