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A Mossbauer study of In-Fe2O3/HZSM-5 catalysts for the selective catalytic reduction of NO by methane
Wang, XD; Zhao, XQ; Shen, JY; Sun, XY; Zhang, T; Lin, LW
Source PublicationPHYSICAL CHEMISTRY CHEMICAL PHYSICS
2002
DOI10.1039/b110515a
Volume4Issue:12Pages:2846-2851
Indexed BySCI
SubtypeArticle
WOS HeadingsScience & Technology ; Physical Sciences
WOS SubjectChemistry, Physical ; Physics, Atomic, Molecular & Chemical
WOS Research AreaChemistry ; Physics
WOS KeywordTEMPERATURE-PROGRAMMED REDUCTION ; FISCHER-TROPSCH CATALYSTS ; SUPPORTED IRON CATALYSTS ; X-RAY-DIFFRACTION ; FE/ZSM-5 CATALYSTS ; NITROGEN MONOXIDE ; EXCESS OXYGEN ; SPECTROSCOPY ; OXIDE ; DURABILITY
AbstractThe selective catalytic reduction of NO by CH4 was compared over In-Fe2O3/HZSM-5 catalysts prepared by impregnation and co-impregnation methods. It was found that the catalyst preparation method greatly affected the catalyst activity. The impregnated catalyst was very active, but the co-impregnated one showed poor activity. The In Fe2O3/HZSM-5 catalysts were investigated by Mossbauer spectroscopy. The results showed that indium cations entered into the iron oxide lattice in the co-impregnated catalyst, while the impregnated catalyst exhibited a more stable structure, when both of the catalysts were treated severely in the reaction atmosphere. Characterization by means of combined in situ temperature programmed reduction (TPR)- Mossbauer spectroscopy further revealed that the performances of the two catalysts were different in the TPR processes.
Language英语
URL查看原文
WOS IDWOS:000176246700054
Citation statistics
Cited Times:15[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/83147
Collection中国科学院大连化学物理研究所
Affiliation1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
2.Nanjing Univ, Dept Chem, Nanjing 210093, Peoples R China
Recommended Citation
GB/T 7714
Wang, XD,Zhao, XQ,Shen, JY,et al. A Mossbauer study of In-Fe2O3/HZSM-5 catalysts for the selective catalytic reduction of NO by methane[J]. PHYSICAL CHEMISTRY CHEMICAL PHYSICS,2002,4(12):2846-2851.
APA Wang, XD,Zhao, XQ,Shen, JY,Sun, XY,Zhang, T,&Lin, LW.(2002).A Mossbauer study of In-Fe2O3/HZSM-5 catalysts for the selective catalytic reduction of NO by methane.PHYSICAL CHEMISTRY CHEMICAL PHYSICS,4(12),2846-2851.
MLA Wang, XD,et al."A Mossbauer study of In-Fe2O3/HZSM-5 catalysts for the selective catalytic reduction of NO by methane".PHYSICAL CHEMISTRY CHEMICAL PHYSICS 4.12(2002):2846-2851.
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