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题名: Tensor density matrix theory for determining population and alignment of symmetric top molecule using rotationally unresolved fluorescence
作者: Cong, SL;  Han, KL;  Lou, NQ
刊名: MOLECULAR PHYSICS
发表日期: 2000-02-10
卷: 98, 期:3, 页:139-147
收录类别: SCI
文章类型: Article
部门归属: 11
项目归属: 1101
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Physics, Atomic, Molecular & Chemical
研究领域[WOS]: Physics
英文摘要: General expressions used for transforming raw laser-induced fluorescence (LIF) intensity into the population and alignment parameters of a symmetric top molecule are derived by employing the density matrix approach. The molecular population and alignment are described by molecular state multipoles. The results are presented for a general excitation-detection geometry and then applied to some special geometries. In general cases, the LIF intensity is a complex function of the initial molecular state multipoles, the dynamic factors and the excitation-detection geometrical factors. It contains a population and 14 alignment multipoles. How to extract all initial state multipoles from the rotationally unresolved emission LIF intensity is discussed in detail.
关键词[WOS]: LASER TECHNIQUES ;  ENERGY-TRANSFER ;  CHEMILUMINESCENT REACTION ;  STATE ;  POLARIZATION ;  PHOTODISSOCIATION ;  ORIENTATION ;  2-PHOTON ;  PRODUCTS ;  CD3I
语种: 英语
原文出处: 查看原文
WOS记录号: WOS:000085028700003
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/85365
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Acad Sinica, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China
2.Dalian Univ Technol, Dept Phys, Dalian 116023, Peoples R China

Recommended Citation:
Cong, SL,Han, KL,Lou, NQ. Tensor density matrix theory for determining population and alignment of symmetric top molecule using rotationally unresolved fluorescence[J]. MOLECULAR PHYSICS,2000,98(3):139-147.
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