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题名: Theoretical study of determining orientation and alignment of symmetric top molecule using laser-induced fluorescence
作者: Cong, SL;  Han, KL;  Lou, NQ
关键词: laser-induced fluorescence ;  orientation ;  alignment
刊名: SCIENCE IN CHINA SERIES B-CHEMISTRY
发表日期: 2000-10-01
卷: 43, 期:5, 页:485-495
收录类别: SCI
文章类型: Article
部门归属: 11
项目归属: 1101
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Multidisciplinary
研究领域[WOS]: Chemistry
英文摘要: General expressions used for extracting the orientation and alignment parameters of a symmetric top molecule from laser-induced fluorescence (LIF) intensity are derived by employing the density matrix approach. The molecular orientation and alignment are described by molecular state multipoles. Excitation and detection are circularly and linearly polarized lights, respectively. In general cases, the LIF intensity is a complex function of the initial molecular state multipoles, the dynamic factors and the excitation-detection geometrical factors. It contains a population, ten orientation and fourteen alignment multipoles. The problem of how to extract the initial molecular state multipoles from the resolved LIF intensity is discussed.
关键词[WOS]: 2-PHOTON NONRESONANT EXCITATION ;  POPULATION
语种: 英语
原文出处: 查看原文
WOS记录号: WOS:000165164300005
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/85373
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China
2.Dalian Univ Technol, Dept Phys, Dalian 116023, Peoples R China

Recommended Citation:
Cong, SL,Han, KL,Lou, NQ. Theoretical study of determining orientation and alignment of symmetric top molecule using laser-induced fluorescence[J]. SCIENCE IN CHINA SERIES B-CHEMISTRY,2000,43(5):485-495.
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