DICP OpenIR
High-throughput screening of HZSM-5 supported metal-oxides catalysts for the coupling of methane with CO to benzene and naphthalene
Wang, H; Liu, ZM; Shen, JH; Liu, HC; Zhang, JL; Liu ZM(刘中民); Liu ZM(刘中民)
KeywordCo Coupling High-throughput Screening Methane Zn/hzsm-5
Source PublicationCATALYSIS COMMUNICATIONS
2005-05-01
ISSN1566-7367
DOI10.1016/j.catcom.2005.02.008
Volume6Issue:5Pages:343-346
Indexed BySCI
SubtypeArticle
Department8
Funding Project803
Contribution Rank1;1
WOS HeadingsScience & Technology ; Physical Sciences
WOS SubjectChemistry, Physical
WOS Research AreaChemistry
WOS KeywordZEOLITE CATALYSTS ; MO/HZSM-5 CATALYSTS ; ACTIVATION ; DEHYDROCONDENSATION ; AROMATIZATION
AbstractHigh-throughput screening of HZSM-5 supported metal-oxides catalysts were carried out for the coupling reaction of methane with CO to aromatics in a multi-stream reactor system. Zn/HZSM-5 and Mo/HZSM-5 were observed to be rather effective for the catalytic formation of aromatics from the coupling reaction of methane with CO. Temperature-programmed reaction has further proven the efficiency of the coupling of methane and CO over Zn/HZSM-5 catalyst. The results were also validated in a conventional fixed-bed reactor coupled with GC. The results propose that the coupling methane with CO toward benzene and naphthalene can be catalyzed by Zn/HZSM-5 at 500 ° C. Both methane and CO are needed for the formation of reactive coke on the catalyst, and the reactive coke may be the initial product in the producing of hydrocarbons. © 2005 Elsevier B.V. All rights reserved.
Language英语
URL查看原文
WOS IDWOS:000228936300005
Citation statistics
Cited Times:3[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/92197
Collection中国科学院大连化学物理研究所
Corresponding AuthorLiu ZM(刘中民); Liu ZM(刘中民)
AffiliationChinese Acad Sci, Dalian Inst Chem Phys, Nat Gas Utilizat & Appl Catalylsis Lab, Dalian 116023, Peoples R China
Recommended Citation
GB/T 7714
Wang, H,Liu, ZM,Shen, JH,et al. High-throughput screening of HZSM-5 supported metal-oxides catalysts for the coupling of methane with CO to benzene and naphthalene[J]. CATALYSIS COMMUNICATIONS,2005,6(5):343-346.
APA Wang, H.,Liu, ZM.,Shen, JH.,Liu, HC.,Zhang, JL.,...&刘中民.(2005).High-throughput screening of HZSM-5 supported metal-oxides catalysts for the coupling of methane with CO to benzene and naphthalene.CATALYSIS COMMUNICATIONS,6(5),343-346.
MLA Wang, H,et al."High-throughput screening of HZSM-5 supported metal-oxides catalysts for the coupling of methane with CO to benzene and naphthalene".CATALYSIS COMMUNICATIONS 6.5(2005):343-346.
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