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High-throughput screening of HZSM-5 supported metal-oxides catalysts for the coupling of methane with CO to benzene and naphthalene
Wang, H; Liu, ZM; Shen, JH; Liu, HC; Zhang, JL; Liu ZM(刘中民); Liu ZM(刘中民)
关键词Co Coupling High-throughput Screening Methane Zn/hzsm-5
刊名CATALYSIS COMMUNICATIONS
2005-05-01
ISSN1566-7367
DOI10.1016/j.catcom.2005.02.008
6期:5页:343-346
收录类别SCI
文章类型Article
部门归属8
项目归属803
产权排名1;1
WOS标题词Science & Technology ; Physical Sciences
类目[WOS]Chemistry, Physical
研究领域[WOS]Chemistry
关键词[WOS]ZEOLITE CATALYSTS ; MO/HZSM-5 CATALYSTS ; ACTIVATION ; DEHYDROCONDENSATION ; AROMATIZATION
英文摘要High-throughput screening of HZSM-5 supported metal-oxides catalysts were carried out for the coupling reaction of methane with CO to aromatics in a multi-stream reactor system. Zn/HZSM-5 and Mo/HZSM-5 were observed to be rather effective for the catalytic formation of aromatics from the coupling reaction of methane with CO. Temperature-programmed reaction has further proven the efficiency of the coupling of methane and CO over Zn/HZSM-5 catalyst. The results were also validated in a conventional fixed-bed reactor coupled with GC. The results propose that the coupling methane with CO toward benzene and naphthalene can be catalyzed by Zn/HZSM-5 at 500 ° C. Both methane and CO are needed for the formation of reactive coke on the catalyst, and the reactive coke may be the initial product in the producing of hydrocarbons. © 2005 Elsevier B.V. All rights reserved.
语种英语
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WOS记录号WOS:000228936300005
引用统计
被引频次:3[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/92197
专题中国科学院大连化学物理研究所
通讯作者Liu ZM(刘中民); Liu ZM(刘中民)
作者单位Chinese Acad Sci, Dalian Inst Chem Phys, Nat Gas Utilizat & Appl Catalylsis Lab, Dalian 116023, Peoples R China
推荐引用方式
GB/T 7714
Wang, H,Liu, ZM,Shen, JH,et al. High-throughput screening of HZSM-5 supported metal-oxides catalysts for the coupling of methane with CO to benzene and naphthalene[J]. CATALYSIS COMMUNICATIONS,2005,6(5):343-346.
APA Wang, H.,Liu, ZM.,Shen, JH.,Liu, HC.,Zhang, JL.,...&刘中民.(2005).High-throughput screening of HZSM-5 supported metal-oxides catalysts for the coupling of methane with CO to benzene and naphthalene.CATALYSIS COMMUNICATIONS,6(5),343-346.
MLA Wang, H,et al."High-throughput screening of HZSM-5 supported metal-oxides catalysts for the coupling of methane with CO to benzene and naphthalene".CATALYSIS COMMUNICATIONS 6.5(2005):343-346.
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