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Mixed reforming of heptane to syngas in the Ba0.5Sr0.5Co0.8Fe0.2O3 membrane reactor
Zhu, WL; Han, W; Xiong, GX; Yang, WS; Xiong GX(熊国兴); Xiong GX(熊国兴)
关键词Membrane Reactor Mixed Reforming Heptane Syngas Hydrogen Production
刊名CATALYSIS TODAY
2005-06-30
DOI10.1016/j.cattod.2005.03.072
104期:2-4页:149-153
收录类别ISTP ; SCI
文章类型Article
部门归属5
项目归属504
产权排名1;1
WOS标题词Science & Technology ; Physical Sciences ; Technology
类目[WOS]Chemistry, Applied ; Chemistry, Physical ; Engineering, Chemical
研究领域[WOS]Chemistry ; Engineering
关键词[WOS]PARTIAL OXIDATION ; METHANE ; STABILITY ; CATALYST ; ETHANE
英文摘要Fuel cells are recognized as the most promising new power generation technology, but hydrogen supply is still a problem. In our previous work, we have developed a LiLaNiO/gamma-Al2O3 catalyst, which is excellent not only for partial oxidation of hydrocarbons, but also for steam reforming and autothermal reforming. However, the reaction needs pure oxygen or air as oxidant. We have developed a dense oxygen permeable membrane Ba0.5Sr0.5Co0.8Fe0.2O3 which has an oxygen permeation flux around 11.5 ml/cm(2) min at reaction conditions. Therefore, this work is to combine the oxygen permeable membrane with the catalyst LiLaNiO/gamma-Al2O3 in a membrane reactor for hydrogen production by mixed reforming of heptane. Under optimized reaction conditions, a heptane conversion of 100%, a CO selectivity of 91-93% and a H-2 selectivity of 95-97% have been achieved. (c) 2005 Elsevier B.V. All rights reserved.
语种英语
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WOS记录号WOS:000230204100008
引用统计
被引频次:25[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/92299
专题中国科学院大连化学物理研究所
通讯作者Xiong GX(熊国兴); Xiong GX(熊国兴)
作者单位Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
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Zhu, WL,Han, W,Xiong, GX,et al. Mixed reforming of heptane to syngas in the Ba0.5Sr0.5Co0.8Fe0.2O3 membrane reactor[J]. CATALYSIS TODAY,2005,104(2-4):149-153.
APA Zhu, WL,Han, W,Xiong, GX,Yang, WS,熊国兴,&熊国兴.(2005).Mixed reforming of heptane to syngas in the Ba0.5Sr0.5Co0.8Fe0.2O3 membrane reactor.CATALYSIS TODAY,104(2-4),149-153.
MLA Zhu, WL,et al."Mixed reforming of heptane to syngas in the Ba0.5Sr0.5Co0.8Fe0.2O3 membrane reactor".CATALYSIS TODAY 104.2-4(2005):149-153.
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