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Mixed reforming of heptane to syngas in the Ba0.5Sr0.5Co0.8Fe0.2O3 membrane reactor
Zhu, WL; Han, W; Xiong, GX; Yang, WS; Xiong GX(熊国兴); Xiong GX(熊国兴)
KeywordMembrane Reactor Mixed Reforming Heptane Syngas Hydrogen Production
Source PublicationCATALYSIS TODAY
2005-06-30
DOI10.1016/j.cattod.2005.03.072
Volume104Issue:2-4Pages:149-153
Indexed ByISTP ; SCI
SubtypeArticle
Department5
Funding Project504
Contribution Rank1;1
WOS HeadingsScience & Technology ; Physical Sciences ; Technology
WOS SubjectChemistry, Applied ; Chemistry, Physical ; Engineering, Chemical
WOS Research AreaChemistry ; Engineering
WOS KeywordPARTIAL OXIDATION ; METHANE ; STABILITY ; CATALYST ; ETHANE
AbstractFuel cells are recognized as the most promising new power generation technology, but hydrogen supply is still a problem. In our previous work, we have developed a LiLaNiO/gamma-Al2O3 catalyst, which is excellent not only for partial oxidation of hydrocarbons, but also for steam reforming and autothermal reforming. However, the reaction needs pure oxygen or air as oxidant. We have developed a dense oxygen permeable membrane Ba0.5Sr0.5Co0.8Fe0.2O3 which has an oxygen permeation flux around 11.5 ml/cm(2) min at reaction conditions. Therefore, this work is to combine the oxygen permeable membrane with the catalyst LiLaNiO/gamma-Al2O3 in a membrane reactor for hydrogen production by mixed reforming of heptane. Under optimized reaction conditions, a heptane conversion of 100%, a CO selectivity of 91-93% and a H-2 selectivity of 95-97% have been achieved. (c) 2005 Elsevier B.V. All rights reserved.
Language英语
URL查看原文
WOS IDWOS:000230204100008
Citation statistics
Cited Times:26[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/92299
Collection中国科学院大连化学物理研究所
Corresponding AuthorXiong GX(熊国兴); Xiong GX(熊国兴)
AffiliationChinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
Recommended Citation
GB/T 7714
Zhu, WL,Han, W,Xiong, GX,et al. Mixed reforming of heptane to syngas in the Ba0.5Sr0.5Co0.8Fe0.2O3 membrane reactor[J]. CATALYSIS TODAY,2005,104(2-4):149-153.
APA Zhu, WL,Han, W,Xiong, GX,Yang, WS,熊国兴,&熊国兴.(2005).Mixed reforming of heptane to syngas in the Ba0.5Sr0.5Co0.8Fe0.2O3 membrane reactor.CATALYSIS TODAY,104(2-4),149-153.
MLA Zhu, WL,et al."Mixed reforming of heptane to syngas in the Ba0.5Sr0.5Co0.8Fe0.2O3 membrane reactor".CATALYSIS TODAY 104.2-4(2005):149-153.
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