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Effect of syngas addition on lower alkene production by the oxidative cracking of hexane
Zhu, H; Liu, XB; Li, WZ; Ge, QJ; Xu, HY; Li WZ(李文钊); Li WZ(李文钊)
刊名ENERGY & FUELS
2005-07-01
DOI10.1021/ef050027+
19期:4页:1704-1707
收录类别SCI
文章类型Article
部门归属8
项目归属801
产权排名1;1
WOS标题词Science & Technology ; Technology
类目[WOS]Energy & Fuels ; Engineering, Chemical
研究领域[WOS]Energy & Fuels ; Engineering
关键词[WOS]LIGHT ALKENES ; N-BUTANE ; DEHYDROGENATION ; CATALYSTS ; HYDROCARBONS ; ETHANE ; CYCLOHEXANE ; MOLYBDENA ; ETHYLENE ; PROPANE
英文摘要The lower alkene production by the gas-phase oxidative cracking (GOC) or catalytic oxidative cracking (COC) of hexane (C6) with added syngas was investigated. The addition of syngas to the COC process could effectively enhance the selectivity to lower alkenes and decrease the selectivity to COx, because of the preferential reaction between O-2 with H-2 contained in the syngas, whereas it has little effect on the conversion of C6 and product distribution in the GOC process. The high selectivity to lower alkenes of 70% and low selectivity to CO, of 6% at C6 conversion of 66% were achieved over 0.1% Pt/MgAl2O4 catalyst. The COC process of C6 combined with the syngas in the feed could directly produce a gas mixture of lower alkenes, H-2, and CO, which usually is a suitable feedstock for the hydroformylation process.
语种英语
原文出处查看原文
WOS记录号WOS:000230706200065
引用统计
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/92377
专题中国科学院大连化学物理研究所
通讯作者Li WZ(李文钊); Li WZ(李文钊)
作者单位Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
推荐引用方式
GB/T 7714
Zhu, H,Liu, XB,Li, WZ,et al. Effect of syngas addition on lower alkene production by the oxidative cracking of hexane[J]. ENERGY & FUELS,2005,19(4):1704-1707.
APA Zhu, H.,Liu, XB.,Li, WZ.,Ge, QJ.,Xu, HY.,...&李文钊.(2005).Effect of syngas addition on lower alkene production by the oxidative cracking of hexane.ENERGY & FUELS,19(4),1704-1707.
MLA Zhu, H,et al."Effect of syngas addition on lower alkene production by the oxidative cracking of hexane".ENERGY & FUELS 19.4(2005):1704-1707.
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