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题名: Reaction path for oxidation of ethylene to acetic acid over Pd/WO3-ZrO2 in the presence of water
作者: Chu, WL;  Ooka, Y;  Kamiya, Y;  Okuhara, T
通讯作者: 楚文玲
关键词: ethylene oxidation ;  acetic acid ;  acetaldehyde ;  reaction path ;  Pd/WO3-ZrO2 ;  Wacker-type reaction
刊名: CATALYSIS LETTERS
发表日期: 2005-06-01
DOI: 10.1007/s10562-005-4896-0
卷: 101, 期:3-4, 页:225-228
收录类别: SCI
文章类型: Article
部门归属: 5
项目归属: 504
产权排名: 2;1
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Physical
研究领域[WOS]: Chemistry
英文摘要: Pd-supported on WO3-ZrO2 (W/Zr atomic ratio=0.2) calcined at 1073 K was found to be highly active and selective for gas-phase oxidation of ethylene to acetic acid in the presence of water at 423 K and 0.6 MPa. Contact time dependence demonstrated that acetic acid is formed via acetaldehyde formed by a Wacker-type reaction, not through ethanol by hydration of ethylene.
语种: 英语
原文出处: 查看原文
WOS记录号: WOS:000229511400016
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/93295
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Hokkaido Univ, Grad Sch Environm Earth Sci, Sapporo, Hokkaido 0600810, Japan
2.Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China

Recommended Citation:
Chu, WL,Ooka, Y,Kamiya, Y,et al. Reaction path for oxidation of ethylene to acetic acid over Pd/WO3-ZrO2 in the presence of water[J]. CATALYSIS LETTERS,2005,101(3-4):225-228.
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