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题名: The observation of quantum bottleneck states
作者: Skodje, RT;  Yang, XM
通讯作者: Rex T.Skodje
刊名: INTERNATIONAL REVIEWS IN PHYSICAL CHEMISTRY
发表日期: 2004-04-01
DOI: 10.1080/01442350412331284616
卷: 23, 期:2, 页:253-287
收录类别: SCI
文章类型: Review
部门归属: 11
项目归属: 1102
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Physical ;  Physics, Atomic, Molecular & Chemical
研究领域[WOS]: Chemistry ;  Physics
英文摘要: The concept of quantum bottleneck states near reaction barriers is essential to the elucidation of chemical reaction rates and reaction dynamics. Recent studies of the dynamics of simple gas-phase chemical reactions have revealed that the transition state controls the detailed observable characteristics of a reaction to a far greater degree than was generally imagined. However, observation of such quantum bottleneck states is extremely difficult. In this article, we provide a review of the current status of observing these quantum bottleneck states in both bimolecular and unimolecular reactions, providing an updated picture of the concept of quantum bottleneck states in chemical reactions.
关键词[WOS]: QUANTIZED TRANSITION-STATES ;  DIFFERENTIAL CROSS-SECTIONS ;  HYDROGEN-EXCHANGE REACTION ;  CHEMICAL-REACTION ;  REACTIVE SCATTERING ;  UNIMOLECULAR DECOMPOSITION ;  REACTION PROBABILITIES ;  SPECTRAL QUANTIZATION ;  REACTION DYNAMICS ;  MOLECULAR-BEAM
语种: 英语
原文出处: 查看原文
WOS记录号: WOS:000224279800003
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/97213
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA
2.Acad Sinica, Inst Atom & Mol Sci, Taipei, Taiwan
3.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Liaoning, Peoples R China

Recommended Citation:
Skodje, RT,Yang, XM. The observation of quantum bottleneck states[J]. INTERNATIONAL REVIEWS IN PHYSICAL CHEMISTRY,2004,23(2):253-287.
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