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Hydrogen production from liquid hydrocarbon fuels for PEMFC application
Chen, Yazhong; Xu, Hengyong; Wang, Yuzhong; Jin, Xianglan; Xiong, Guoxing; Xiong GX(熊国兴); Xiong GX(熊国兴)
关键词Liquid Hydrocarbons Prereforming Autothermal Reforming Distributed Air Feed Nickel Catalyst Pd Membrane
刊名FUEL PROCESSING TECHNOLOGY
2006-11-01
DOI10.1016/j.fuproc.2006.07.007
87期:11页:971-978
收录类别SCI
文章类型Article
部门归属8,5
项目归属801,504
产权排名1;1
WOS标题词Science & Technology ; Physical Sciences ; Technology
类目[WOS]Chemistry, Applied ; Energy & Fuels ; Engineering, Chemical
研究领域[WOS]Chemistry ; Energy & Fuels ; Engineering
关键词[WOS]GAS-PRODUCTION ; CELL SYSTEMS ; SEPARATION ; CATALYSTS
英文摘要Lack of efficient hydrogen storage intermediate has boosted the development of fuel processor or economic onsite hydrogen production techniques for application to proton exchange membrane fuel cell promptly. Aiming to develop onsite hydrogen production techniques for proton exchange membrane fuel cell application using nickel-based reforming catalysts and stainless steel reactors, in this paper, a novel process for H-2 production from liquid hydrocarbon fuels was proposed and experimentally demonstrated on a lab scale. The main operations involved prereforming, autothermal reforming, high temperature water gas shift, low temperature water gas shift and H-2 enrichment by Pd membrane. The results indicated that prereforming introduction prior to autothermal reforming suppressed undesired gas phase reactions efficiently and made reforming reactions perform catalytically and smoothly, which was confirmed by a stable 500 h time-on-stream test of both prereforming and autothermal reforming catalysts. The air distributed feed applied in autothermal reforming reactor coupled the endothermic steam reforming and exothermic catalytic combustion reactions over the catalyst closely, maintaining an appropriate temperature distribution curve for autothermal reforming catalyst bed. During the process of H-2 enrichment by highly H-2 permeable Pd composite membrane, concentration polarization played an important role. (C) 2006 Elsevier B.V. All rights reserved.
语种英语
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WOS记录号WOS:000241960300004
引用统计
被引频次:20[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/97651
专题中国科学院大连化学物理研究所
通讯作者Xiong GX(熊国兴); Xiong GX(熊国兴)
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, Appl Catalysis Lab, Dalian 116023, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
3.Res Inst Daqing Petrohem Co, Daqing 163000, Peoples R China
推荐引用方式
GB/T 7714
Chen, Yazhong,Xu, Hengyong,Wang, Yuzhong,et al. Hydrogen production from liquid hydrocarbon fuels for PEMFC application[J]. FUEL PROCESSING TECHNOLOGY,2006,87(11):971-978.
APA Chen, Yazhong.,Xu, Hengyong.,Wang, Yuzhong.,Jin, Xianglan.,Xiong, Guoxing.,...&熊国兴.(2006).Hydrogen production from liquid hydrocarbon fuels for PEMFC application.FUEL PROCESSING TECHNOLOGY,87(11),971-978.
MLA Chen, Yazhong,et al."Hydrogen production from liquid hydrocarbon fuels for PEMFC application".FUEL PROCESSING TECHNOLOGY 87.11(2006):971-978.
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