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Pd-Zn/Cu-Zn-Al catalysts prepared for methanol oxidation reforming in microchannel reactors
Chen, Guangwen; Li, Shuhan; Yuan, Quan; Chen GW(陈光文); Chen GW(陈光文)
关键词Microchannel Microstructured Reactor Wall Coating Oxidation Reforming Microreactor
刊名CATALYSIS TODAY
2007-01-30
DOI10.1016/j.cattod.2006.07.004
120期:1页:63-70
收录类别ISTP ; SCI
文章类型Article
部门归属9
项目归属903
产权排名1;1
WOS标题词Science & Technology ; Physical Sciences ; Technology
类目[WOS]Chemistry, Applied ; Chemistry, Physical ; Engineering, Chemical
研究领域[WOS]Chemistry ; Engineering
关键词[WOS]HYDROGEN-PRODUCTION ; FUEL-CELL ; MICROSTRUCTURED REACTORS ; PD/ZNO CATALYST ; STEAM ; TECHNOLOGY
英文摘要Methanol oxidation reforming is an important reaction in the process of hydrogen generation for PEMFC. In this paper, we report the wall coated catalysts in a microchannel reactor for methanol oxidation reforming. The preparation method of the wall coating catalyst was studied in detail, i.e., the sol-get and solution-coating techniques. To prepare the catalysts for methanol oxidation reforming, the washing-coating layer of CuZnAl was prepared by the sol-gel technique, and then the active layer was coated on it by solution-coating technique with emulsion colloid containing Pd-ZnO particles. Both the supporting layer and catalyst on the stainless steel foils were characterized by scanning electron microscopy (SEM) and X-ray diffraction (XRD). The formed wash-coating layer with ordered arrays of petaloid microcrystallites in layer surface and Pd-Zn alloy crystal phase can be clearly observed. The reaction experimental results indicated that the catalyst prepared have high activity and relatively high stability. (c) 2006 Elsevier B.V. All rights reserved.
语种英语
原文出处查看原文
WOS记录号WOS:000242378900008
引用统计
被引频次:31[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/98415
专题中国科学院大连化学物理研究所
通讯作者Chen GW(陈光文); Chen GW(陈光文)
作者单位Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
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GB/T 7714
Chen, Guangwen,Li, Shuhan,Yuan, Quan,et al. Pd-Zn/Cu-Zn-Al catalysts prepared for methanol oxidation reforming in microchannel reactors[J]. CATALYSIS TODAY,2007,120(1):63-70.
APA Chen, Guangwen,Li, Shuhan,Yuan, Quan,陈光文,&陈光文.(2007).Pd-Zn/Cu-Zn-Al catalysts prepared for methanol oxidation reforming in microchannel reactors.CATALYSIS TODAY,120(1),63-70.
MLA Chen, Guangwen,et al."Pd-Zn/Cu-Zn-Al catalysts prepared for methanol oxidation reforming in microchannel reactors".CATALYSIS TODAY 120.1(2007):63-70.
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