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Integrated one-step PEMFC-grade hydrogen production from liquid hydrocarbons using Pd membrane reactor
Chen, Yazhong; Wang, Yuzhong; Xu, Hengyong; Xiong, Guoxing; Xu HY(徐恒泳); Xu HY(徐恒泳)
刊名INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
2007-08-15
DOI10.1021/ie070150j
46期:17页:5510-5515
收录类别SCI
文章类型Article
部门归属8,5
项目归属801,504
产权排名1;1
WOS标题词Science & Technology ; Technology
类目[WOS]Engineering, Chemical
研究领域[WOS]Engineering
关键词[WOS]DEHYDROGENATION ; TEMPERATURE ; METHANE ; CATALYSTS
英文摘要A process of hydrogen production for application to proton exchange membrane fuel cells (PEMFC), a kind of efficient and almost zero-emission power-generation device, was developed by integrating the reactions during the steam reforming of multicomponent liquid hydrocarbon fuels and hydrogen enrichment in a Pd membrane reactor. A highly hydrogen permeable, permselective Pd composite membrane, and an active catalyst for steam reforming of not only higher hydrocarbons but also of methane at temperatures lower than 823 K, made one-step hydrogen production from steam reforming of liquid hydrocarbons in a membrane reactor feasible near practical working conditions. Furthermore, a theoretical energy balance calculation showed that the membrane not only separated hydrogen but also adjusted the selectivities of products, which could be applied to achieve autothermal operation, e. g., catalytic combustion of the reformate from the retentate side of the Pd membrane could provide the energy for the endothermic steam reforming reactions in such a fuel processor system.
语种英语
原文出处查看原文
WOS记录号WOS:000248657700006
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被引频次:7[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://cas-ir.dicp.ac.cn/handle/321008/99575
专题中国科学院大连化学物理研究所
通讯作者Xu HY(徐恒泳); Xu HY(徐恒泳)
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
2.Nanjing Inst Chem Technol, Coll Chem & Chem Engn, Membrane Sci Res Ctr, Nanjing 210009, JiangSu, Peoples R China
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GB/T 7714
Chen, Yazhong,Wang, Yuzhong,Xu, Hengyong,et al. Integrated one-step PEMFC-grade hydrogen production from liquid hydrocarbons using Pd membrane reactor[J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,2007,46(17):5510-5515.
APA Chen, Yazhong,Wang, Yuzhong,Xu, Hengyong,Xiong, Guoxing,徐恒泳,&徐恒泳.(2007).Integrated one-step PEMFC-grade hydrogen production from liquid hydrocarbons using Pd membrane reactor.INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,46(17),5510-5515.
MLA Chen, Yazhong,et al."Integrated one-step PEMFC-grade hydrogen production from liquid hydrocarbons using Pd membrane reactor".INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 46.17(2007):5510-5515.
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