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Integrated one-step PEMFC-grade hydrogen production from liquid hydrocarbons using Pd membrane reactor
Chen, Yazhong; Wang, Yuzhong; Xu, Hengyong; Xiong, Guoxing; Xu HY(徐恒泳); Xu HY(徐恒泳)
Source PublicationINDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
2007-08-15
DOI10.1021/ie070150j
Volume46Issue:17Pages:5510-5515
Indexed BySCI
SubtypeArticle
Department8,5
Funding Project801,504
Contribution Rank1;1
WOS HeadingsScience & Technology ; Technology
WOS SubjectEngineering, Chemical
WOS Research AreaEngineering
WOS KeywordDEHYDROGENATION ; TEMPERATURE ; METHANE ; CATALYSTS
AbstractA process of hydrogen production for application to proton exchange membrane fuel cells (PEMFC), a kind of efficient and almost zero-emission power-generation device, was developed by integrating the reactions during the steam reforming of multicomponent liquid hydrocarbon fuels and hydrogen enrichment in a Pd membrane reactor. A highly hydrogen permeable, permselective Pd composite membrane, and an active catalyst for steam reforming of not only higher hydrocarbons but also of methane at temperatures lower than 823 K, made one-step hydrogen production from steam reforming of liquid hydrocarbons in a membrane reactor feasible near practical working conditions. Furthermore, a theoretical energy balance calculation showed that the membrane not only separated hydrogen but also adjusted the selectivities of products, which could be applied to achieve autothermal operation, e. g., catalytic combustion of the reformate from the retentate side of the Pd membrane could provide the energy for the endothermic steam reforming reactions in such a fuel processor system.
Language英语
URL查看原文
WOS IDWOS:000248657700006
Citation statistics
Cited Times:7[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://cas-ir.dicp.ac.cn/handle/321008/99575
Collection中国科学院大连化学物理研究所
Corresponding AuthorXu HY(徐恒泳); Xu HY(徐恒泳)
Affiliation1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
2.Nanjing Inst Chem Technol, Coll Chem & Chem Engn, Membrane Sci Res Ctr, Nanjing 210009, JiangSu, Peoples R China
Recommended Citation
GB/T 7714
Chen, Yazhong,Wang, Yuzhong,Xu, Hengyong,et al. Integrated one-step PEMFC-grade hydrogen production from liquid hydrocarbons using Pd membrane reactor[J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,2007,46(17):5510-5515.
APA Chen, Yazhong,Wang, Yuzhong,Xu, Hengyong,Xiong, Guoxing,徐恒泳,&徐恒泳.(2007).Integrated one-step PEMFC-grade hydrogen production from liquid hydrocarbons using Pd membrane reactor.INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,46(17),5510-5515.
MLA Chen, Yazhong,et al."Integrated one-step PEMFC-grade hydrogen production from liquid hydrocarbons using Pd membrane reactor".INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 46.17(2007):5510-5515.
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