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题名: Integrated one-step PEMFC-grade hydrogen production from liquid hydrocarbons using Pd membrane reactor
作者: Chen, Yazhong;  Wang, Yuzhong;  Xu, Hengyong;  Xiong, Guoxing
通讯作者: 徐恒泳
刊名: INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
发表日期: 2007-08-15
DOI: 10.1021/ie070150j
卷: 46, 期:17, 页:5510-5515
收录类别: SCI
文章类型: Article
部门归属: 8,5
项目归属: 801,504
产权排名: 1;1
WOS标题词: Science & Technology ;  Technology
类目[WOS]: Engineering, Chemical
研究领域[WOS]: Engineering
英文摘要: A process of hydrogen production for application to proton exchange membrane fuel cells (PEMFC), a kind of efficient and almost zero-emission power-generation device, was developed by integrating the reactions during the steam reforming of multicomponent liquid hydrocarbon fuels and hydrogen enrichment in a Pd membrane reactor. A highly hydrogen permeable, permselective Pd composite membrane, and an active catalyst for steam reforming of not only higher hydrocarbons but also of methane at temperatures lower than 823 K, made one-step hydrogen production from steam reforming of liquid hydrocarbons in a membrane reactor feasible near practical working conditions. Furthermore, a theoretical energy balance calculation showed that the membrane not only separated hydrogen but also adjusted the selectivities of products, which could be applied to achieve autothermal operation, e. g., catalytic combustion of the reformate from the retentate side of the Pd membrane could provide the energy for the endothermic steam reforming reactions in such a fuel processor system.
关键词[WOS]: DEHYDROGENATION ;  TEMPERATURE ;  METHANE ;  CATALYSTS
语种: 英语
原文出处: 查看原文
WOS记录号: WOS:000248657700006
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/99575
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China
2.Nanjing Inst Chem Technol, Coll Chem & Chem Engn, Membrane Sci Res Ctr, Nanjing 210009, JiangSu, Peoples R China

Recommended Citation:
Chen, Yazhong,Wang, Yuzhong,Xu, Hengyong,et al. Integrated one-step PEMFC-grade hydrogen production from liquid hydrocarbons using Pd membrane reactor[J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,2007,46(17):5510-5515.
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