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题名: Production of hydrogen peroxide by the reaction of hydroxylamine and molecular oxygen over activated carbons
作者: Song, Wei1;  Li, Juan1;  Liu, Junlong1;  Shen, Wenjie1
通讯作者: 申文杰
关键词: in situ production ;  hydrogen peroxide ;  hydroxylamine ;  oxygen ;  activated carbon
刊名: CATALYSIS COMMUNICATIONS
发表日期: 2008-03-20
DOI: 10.1016/j.catcom.2007.09.006
卷: 9, 期:5, 页:831-836
收录类别: SCI
文章类型: Article
部门归属: 5
项目归属: 501
产权排名: 1;1
WOS标题词: Science & Technology ;  Physical Sciences
类目[WOS]: Chemistry, Physical
研究领域[WOS]: Chemistry
英文摘要: In situ production of hydrogen peroxide was achieved by the reaction of hydroxylamine and molecular oxygen over reusable activated carbon catalysts at ambient temperature with environmentally benign by-products (nitrogen and water). The yield of hydrogen peroxide was about 46% with the concentration of 0.39 wt% (114 mmol/L). Temperature-programmed desorption analysis and Fourier transformation infrared spectroscopy revealed that the oxygen-containing species, especially quinone/semiquinone-like structures, on the surface of activated carbon played a crucial role in the generation of H2O2, probably through the effective activation of oxygen molecule. (c) 2007 Elsevier B.V. All rights reserved.
关键词[WOS]: IN-SITU GENERATION ;  PD/AL2O3 CATALYST ;  NONAQUEOUS MEDIUM ;  REDUCTION ;  OXIDATION ;  DIOXYGEN ;  COMPLEXES ;  CHEMISTRY ;  MEMBRANE ;  BENZENE
语种: 英语
原文出处: 查看原文
WOS记录号: WOS:000253450900051
Citation statistics: 
内容类型: 期刊论文
URI标识: http://cas-ir.dicp.ac.cn/handle/321008/99945
Appears in Collections:中国科学院大连化学物理研究所_期刊论文

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作者单位: 1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China

Recommended Citation:
Song, Wei,Li, Juan,Liu, Junlong,et al. Production of hydrogen peroxide by the reaction of hydroxylamine and molecular oxygen over activated carbons[J]. CATALYSIS COMMUNICATIONS,2008,9(5):831-836.
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